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After condensing the vapors in a cooling tray, a dark\u2010brown bioliquid is obtained. The quality of the thus obtained fast pyrolysis oil has some barriers for its direct use as transportation fuel. Low caloric value, high viscosity, and corrosion are the major challenges for its implementation in conventional engines. There have been sustained efforts to improve the quality of the oil. In this Communication we are reporting a concept on improving the acidic properties by means of a combined catalysis and adsorption approach. We found that fast pyrolysis oil can be upgraded through alcoholysis using n<\/jats:italic>\u2010butanol and tetrahydrofurfuryl alcohol, which are biomass\u2010derived bulk chemicals. The reaction is acid catalyzed whereas water is continuously separated from the condensate mixture through molecular sieve adsorption. 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Behav. Med."],"abstract":"Abstract<\/jats:title>\n Background<\/jats:title>\n Cognitive complaints (e.g., health anxiety and illness disruption) are commonly experienced by patients with coronary heart disease (CHD). While it is known that sex and gender affect health, their influence on cognitive complaints remains unknown. The current study explored sex and gender differences in cognitive complaints during the first month (acute phase) and beyond, up to 2\u00a0years (recovery phase) after percutaneous coronary intervention (PCI).<\/jats:p>\n <\/jats:sec>\n Method<\/jats:title>\n A total of 514 (M<\/jats:italic>age<\/jats:sub>\u2009=\u200964.2\u2009\u00b1\u20098.9, 84.2% male) completed the cognitive scale of the Health Complaints Scale (i.e., overall cognitive complaints, health worry, illness disruption) at baseline, 1, 12, and 24\u00a0months post-PCI. Additional questionnaires to gauge gender identity, traits, and norms were administered in a follow-up study. General linear mixed model analyses were conducted to examine the influence of sex, gender, sex\u2009\u00d7\u2009gender, and covariates on cognitive complaints.<\/jats:p>\n <\/jats:sec>\n Results<\/jats:title>\n Cognitive complaints only decreased in the first month post-PCI (all p<\/jats:italic>\u2009<\u2009.01). There were no clear sex differences. However, gender generally predicted cognitive complaints in the first 2 years post-PCI: masculinity was related to less complaints, whereas feminine individuals reported higher absolute levels of complaints.<\/jats:p>\n <\/jats:sec>\n Conclusion<\/jats:title>\n The current findings reveal that gender is a valuable factor concerning health complaints and indicate the need to further elaborate on the discrepancies between sex and gender in health research.<\/jats:p>\n <\/jats:sec>","DOI":"10.1007\/s12529-024-10333-y","type":"journal-article","created":{"date-parts":[[2024,11,6]],"date-time":"2024-11-06T17:07:00Z","timestamp":1730912820000},"update-policy":"https:\/\/doi.org\/10.1007\/springer_crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["The Influence of Sex and Gender on the Level and Course of Subjective Cognitive Complaints After Percutaneous Coronary Intervention"],"prefix":"10.1007","author":[{"given":"Sophie C. 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Although these errors likely arise in the spatiotemporal integration of the tactile input and information about arm position, the underlying arm position information used in this process is not known. In this study, we tested the contributions of afferent proprioceptive feedback and predictive arm position signals by comparing localization errors during passive vs. active arm movements. In the active trials, participants were instructed to localize a tactile stimulus in the external space that was presented to the index finger near the time of a self-generated arm movement. In the passive trials, each of the active trials was passively replayed in randomized order, using a robotic device. Our results provide evidence that the localization error patterns of the passive trials are similar to the active trials and, moreover, did not lag but rather led the active trials, which suggests that proprioceptive feedback makes an important contribution to tactile localization. To further test which kinematic property of this afferent feedback signal drives the underlying computations, we examined the localization errors with movements that had differently skewed velocity profiles but overall the same displacement. This revealed a difference in the localization patterns, which we explain by a probabilistic model in which temporal uncertainty about the stimulus is converted into a spatial likelihood, depending on the actual velocity of the arm rather than involving an efferent, preprogrammed movement. <\/jats:p> NEW & NOTEWORTHY We show that proprioceptive feedback of arm motion rather than efferent motor signals contributes to tactile localization during an arm movement. Data further show that localization errors depend on arm velocity, not displacement per se, suggesting that instantaneous velocity feedback plays a role in the underlying computations. 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Rev. Research"],"accepted":{"date-parts":[[2025,4,14]]},"abstract":"We study the occurrence of Rydberg atom-ion molecules (RAIMs) in a hybrid atom-ion system with an ion crystal trapped in a Paul trap coupled to Rydberg atoms on its either ends. To assess the feasibility of such a system, we perform a detailed Floquet analysis of the effect of the Paul trap's rf potential on the RAIMs and provide a qualitative analysis of the survival probability based on scaling laws. We conclude that the RAIM survives for sufficiently weak and low-frequency traps. We then use this hybrid system and propose a scheme to utilize the common motional modes of the ion crystal to suppress (blockade) or enhance (antiblockade) the probability of forming two RAIMs at the ends of the chain, replacing the typical blockade radius by the length of the ion crystal.<\/jats:p>","DOI":"10.1103\/physrevresearch.7.l022028","type":"journal-article","created":{"date-parts":[[2025,5,2]],"date-time":"2025-05-02T10:05:57Z","timestamp":1746180357000},"update-policy":"https:\/\/doi.org\/10.1103\/crossmark-policy","source":"Crossref","is-referenced-by-count":0,"title":["Vibrationally coupled Rydberg atom-ion molecules"],"prefix":"10.1103","volume":"7","author":[{"ORCID":"https:\/\/orcid.org\/0009-0006-5361-098X","authenticated-orcid":true,"given":"Ilango","family":"Maran","sequence":"first","affiliation":[{"id":[{"id":"https:\/\/ror.org\/04dkp9463","id-type":"ROR","asserted-by":"publisher"}],"name":"University of Amsterdam"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6157-265X","authenticated-orcid":true,"given":"Liam J.","family":"Bond","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/00zq3ce72","id-type":"ROR","asserted-by":"publisher"}],"name":"QuSoft"},{"id":[{"id":"https:\/\/ror.org\/04dkp9463","id-type":"ROR","asserted-by":"publisher"}],"name":"University of Amsterdam"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0971-6067","authenticated-orcid":true,"given":"Jeremy T.","family":"Young","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/04dkp9463","id-type":"ROR","asserted-by":"publisher"}],"name":"University of Amsterdam"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Arghavan","family":"Safavi-Naini","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/00zq3ce72","id-type":"ROR","asserted-by":"publisher"}],"name":"QuSoft"},{"id":[{"id":"https:\/\/ror.org\/04dkp9463","id-type":"ROR","asserted-by":"publisher"}],"name":"University of Amsterdam"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3466-5719","authenticated-orcid":true,"given":"Rene","family":"Gerritsma","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/04dkp9463","id-type":"ROR","asserted-by":"publisher"}],"name":"University of Amsterdam"},{"id":[{"id":"https:\/\/ror.org\/00zq3ce72","id-type":"ROR","asserted-by":"publisher"}],"name":"QuSoft"}],"role":[{"role":"author","vocabulary":"crossref"}]}],"member":"16","published-online":{"date-parts":[[2025,5,2]]},"reference":[{"key":"PhysRevResearch.7.L022028Cc1R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevResearch.3.023114","type":"journal-article"},{"key":"PhysRevResearch.7.L022028Cc2R1","doi-asserted-by":"publisher","DOI":"10.3390\/atoms9020034","type":"journal-article"},{"key":"PhysRevResearch.7.L022028Cc3R1","doi-asserted-by":"publisher","DOI":"10.1038\/s41586-022-04577-5","type":"journal-article"},{"key":"PhysRevResearch.7.L022028Cc4R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.130.023002","type":"journal-article"},{"key":"PhysRevResearch.7.L022028Cc5R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevA.62.042703","type":"journal-article"},{"key":"PhysRevResearch.7.L022028Cc6R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevA.94.013420","type":"journal-article"},{"key":"PhysRevResearch.7.L022028Cc7R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.118.263201","type":"journal-article"},{"key":"PhysRevResearch.7.L022028Cc8R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.121.193401","type":"journal-article"},{"key":"PhysRevResearch.7.L022028Cc10R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.122.253401","type":"journal-article"},{"key":"PhysRevResearch.7.L022028Cc11R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevA.110.062618","type":"journal-article"},{"key":"PhysRevResearch.7.L022028Cc12R1","doi-asserted-by":"publisher","DOI":"10.1088\/1367-2630\/10\/9\/093009","type":"journal-article"},{"key":"PhysRevResearch.7.L022028Cc14R1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cpc.2020.107814","type":"journal-article"},{"key":"PhysRevResearch.7.L022028Cc16R1","doi-asserted-by":"publisher","DOI":"10.1103\/RevModPhys.75.281","type":"journal-article"},{"key":"PhysRevResearch.7.L022028Cc17R1","doi-asserted-by":"publisher","DOI":"10.1016\/j.physrep.2010.03.002","type":"journal-article"},{"key":"PhysRevResearch.7.L022028Cc18R1","doi-asserted-by":"crossref","DOI":"10.1017\/CBO9780511524530","type":"book","volume-title":"Rydberg Atoms","author":"T. Gallagher","year":"1994"},{"key":"PhysRevResearch.7.L022028Cc19R1","doi-asserted-by":"publisher","DOI":"10.1007\/s100530170275","type":"journal-article"},{"key":"PhysRevResearch.7.L022028Cc20R1","doi-asserted-by":"publisher","DOI":"10.1016\/B978-0-12-408090-4.00004-9","type":"journal-article"},{"key":"PhysRevResearch.7.L022028Cc21R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.106.190501","type":"journal-article"}],"container-title":["Physical Review Research"],"language":"en","link":[{"URL":"https:\/\/link.aps.org\/article\/10.1103\/PhysRevResearch.7.L022028","content-type":"unspecified","content-version":"vor","intended-application":"syndication"},{"URL":"http:\/\/harvest.aps.org\/v2\/journals\/articles\/10.1103\/PhysRevResearch.7.L022028\/fulltext","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2025,8,5]],"date-time":"2025-08-05T16:35:22Z","timestamp":1754411722000},"score":0.0,"resource":{"primary":{"URL":"https:\/\/link.aps.org\/doi\/10.1103\/PhysRevResearch.7.L022028"}},"issued":{"date-parts":[[2025,5,2]]},"references-count":18,"journal-issue":{"issue":"2","published-print":{"date-parts":[[2025,5]]}},"URL":"https:\/\/doi.org\/10.1103\/physrevresearch.7.l022028","relation":{"has-preprint":[{"id-type":"doi","id":"10.48550\/arXiv.2409.13469","asserted-by":"subject"}]},"ISSN":["2643-1564"],"issn-type":[{"type":"electronic","value":"2643-1564"}],"published":{"date-parts":[[2025,5,2]]},"assertion":[{"value":"2024-09-23","name":"date_received","label":"Date Received","group":{"name":"publication_dates","label":"Publication dates"}},{"value":"Published by the American Physical Society","name":"copyright_statement","label":"Copyright statement","group":{"name":"copyright","label":"copyright"}},{"value":"2025","name":"copyright_year","label":"Copyright year","group":{"name":"copyright","label":"copyright"}}],"article-number":"L022028"},{"indexed":{"date-parts":[[2025,8,15]],"date-time":"2025-08-15T00:27:16Z","timestamp":1755217636354,"version":"3.43.0"},"reference-count":97,"publisher":"American Physical Society (APS)","issue":"1","license":[{"start":{"date-parts":[[2025,7,7]],"date-time":"2025-07-07T00:00:00Z","timestamp":1751846400000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"DOI":"10.13039\/501100003246","name":"Nederlandse Organisatie voor Wetenschappelijk Onderzoek","doi-asserted-by":"publisher","award":["17877"],"award-info":[{"award-number":["17877"]}],"id":[{"id":"10.13039\/501100003246","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["journals.aps.org"],"crossmark-restriction":true},"short-container-title":["Phys. Rev. B"],"accepted":{"date-parts":[[2025,5,21]]},"abstract":"The hexagonal Mn<\/a:mi>3<\/a:mn>\u2212<\/a:mo>x<\/a:mi><\/a:mrow><\/a:msub>Fe<\/a:mi>x<\/a:mi><\/a:msub>Sn<\/a:mi><\/a:mrow><\/a:math> compounds possess several desirable properties that make them suitable magnetocaloric materials, including a ferromagnetic (FM)-to-paramagnetic (PM) transition near room temperature and soft magnetic behavior. In this study, we use the melt-spinning technique to explore the Mn-Fe-Sn ternary system. By combining magnetization measurements, M\u00f6ssbauer spectroscopy, neutron diffraction (ND), oriented powder x-ray diffraction, and density functional theory (DFT) calculation, the magnetocaloric effect, spin structures, and the intrinsic magnetic properties of polycrystalline Mn<\/d:mi>3<\/d:mn>\u2212<\/d:mo>x<\/d:mi><\/d:mrow><\/d:msub>Fe<\/d:mi>x<\/d:mi><\/d:msub>Sn<\/d:mi><\/d:mrow><\/d:math> (<\/g:mo>x<\/g:mi>=<\/g:mo>0.8<\/g:mn>\u2212<\/g:mo>1.4<\/g:mn>)<\/g:mo><\/g:mrow><\/g:math> compounds are determined. The FM-to-PM transition temperature T<\/h:mi>C<\/h:mi><\/h:msub><\/h:math> ranges from 253 K (<\/j:mo>x<\/j:mi>=<\/j:mo>0.8<\/j:mn>)<\/j:mo><\/j:mrow><\/j:math> to 394 K (<\/k:mo>x<\/k:mi>=<\/k:mo>1.4<\/k:mn>)<\/k:mo><\/k:mrow><\/k:math>. At low temperature, a spin reorientation at T<\/l:mi>S<\/l:mi><\/l:msub><\/l:math> is observed, where below T<\/n:mi>S<\/n:mi><\/n:msub><\/n:math> a coexistence of FM order with spins along the c<\/p:mi><\/p:math> axis and antiferromagnetic order with spins within the a<\/q:mi>\u2212<\/q:mo>b<\/q:mi><\/q:mrow><\/q:math> plane occurs for x<\/r:mi>=<\/r:mo>0.8<\/r:mn><\/r:mrow><\/r:math> and 1.0. However, for compounds with x<\/s:mi>=<\/s:mo>1.2<\/s:mn><\/s:mrow><\/s:math> and 1.4, only FM order with spins along the c<\/t:mi><\/t:math> axis has been found below T<\/u:mi>S<\/u:mi><\/u:msub><\/u:math>. Above T<\/w:mi>S<\/w:mi><\/w:msub><\/w:math>, the spin structure corresponds to FM order with spins aligned within the a<\/y:mi>\u2212<\/y:mo>b<\/y:mi><\/y:mrow><\/y:math> plane for all compositions. The magnetic moments of Mn and Fe were evaluated using DFT, demonstrating good agreement with the ND results.<\/jats:p>","DOI":"10.1103\/pvjm-jvsr","type":"journal-article","created":{"date-parts":[[2025,5,21]],"date-time":"2025-05-21T13:49:57Z","timestamp":1747835397000},"update-policy":"https:\/\/doi.org\/10.1103\/crossmark-policy","source":"Crossref","is-referenced-by-count":0,"title":["Complex spin structure and magnetic phase transition of \nMn<\/mml:mi>3<\/mml:mn>\u2212<\/mml:mo>x<\/mml:mi><\/mml:mrow><\/mml:msub>Fe<\/mml:mi>x<\/mml:mi><\/mml:msub>Sn<\/mml:mi><\/mml:mrow><\/mml:math>\n alloys"],"prefix":"10.1103","volume":"112","author":[{"ORCID":"https:\/\/orcid.org\/0009-0008-7192-5170","authenticated-orcid":true,"given":"W.","family":"Hanggai","sequence":"first","affiliation":[{"id":[{"id":"https:\/\/ror.org\/02e2c7k09","id-type":"ROR","asserted-by":"publisher"}],"name":"Delft University of Technology"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"O.","family":"Hamutu","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/02e2c7k09","id-type":"ROR","asserted-by":"publisher"}],"name":"Delft University of Technology"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1818-0738","authenticated-orcid":true,"given":"G. A.","family":"de Wijs","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/05wg1m734","id-type":"ROR","asserted-by":"publisher"}],"name":"Radboud University"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5559-9573","authenticated-orcid":true,"given":"I.","family":"Dugulan","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/02e2c7k09","id-type":"ROR","asserted-by":"publisher"}],"name":"Delft University of Technology"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2506-2852","authenticated-orcid":true,"given":"N. 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