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As the atmospheric mixing ratios of methyl chloroform (CH\n                    <jats:sub>3<\/jats:sub>\n                    CCl\n                    <jats:sub>3<\/jats:sub>\n                    ) (MCF), the commonly used OH reference gas, approaches zero, it is important to find alternative approaches to infer atmospheric OH abundance and variability. The lack of global bottom\u2010up emission inventories is the primary obstacle in choosing a MCF alternative. We illustrate that global emissions of long\u2010lived trace gases can be inferred from their observed mixing ratio differences between the Northern Hemisphere (NH) and Southern Hemisphere (SH), given realistic estimates of their NH\u2010SH exchange time, the emission partitioning between the two hemispheres, and the NH versus SH OH abundance ratio. Using the observed long\u2010term trend and emissions derived from the measured hemispheric gradient, the combination of HFC\u201032 (CH\n                    <jats:sub>2<\/jats:sub>\n                    F\n                    <jats:sub>2<\/jats:sub>\n                    ), HFC\u2010134a (CH\n                    <jats:sub>2<\/jats:sub>\n                    FCF\n                    <jats:sub>3<\/jats:sub>\n                    , HFC\u2010152a (CH\n                    <jats:sub>3<\/jats:sub>\n                    CHF\n                    <jats:sub>2<\/jats:sub>\n                    ), and HCFC\u201022 (CHClF\n                    <jats:sub>2<\/jats:sub>\n                    ), instead of a single gas, will be useful as a MCF alternative to infer global and hemispheric OH abundance and trace gas lifetimes. The primary assumption on which this multispecies approach relies is that the OH lifetimes can be estimated by scaling the thermal reaction rates of a reference gas at 272\u00a0K on global and hemispheric scales. Thus, the derived hemispheric and global OH estimates are forced to reconcile the observed trends and gradient for all four compounds simultaneously. However, currently, observations of these gases from the surface networks do not provide more accurate OH abundance estimate than that from MCF.\n                  <\/jats:p>","DOI":"10.1002\/2017jd026926","type":"journal-article","created":{"date-parts":[[2017,10,10]],"date-time":"2017-10-10T06:16:36Z","timestamp":1507616196000},"source":"Crossref","is-referenced-by-count":37,"title":["Deriving Global OH Abundance and Atmospheric Lifetimes for Long\u2010Lived Gases: A Search for CH\n                    <sub>3<\/sub>\n                    CCl\n                    <sub>3<\/sub>\n                    Alternatives"],"prefix":"10.1029","volume":"122","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-8430-0515","authenticated-orcid":false,"given":"Qing","family":"Liang","sequence":"first","affiliation":[{"name":"Atmospheric Chemistry and Dynamics Laboratory NASA Goddard Space Flight Center  Greenbelt Maryland USA"},{"name":"Universities Space Research Association, GESTAR  Columbia Maryland USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6803-4149","authenticated-orcid":false,"given":"Martyn P.","family":"Chipperfield","sequence":"additional","affiliation":[{"name":"National Centre for Earth Observation, School of Earth and Environment University of Leeds  Leeds UK"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Eric L.","family":"Fleming","sequence":"additional","affiliation":[{"name":"Atmospheric Chemistry and Dynamics Laboratory NASA Goddard Space Flight Center  Greenbelt Maryland USA"},{"name":"Science Systems and Applications, Inc  Lanham Maryland USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"N. 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