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Herein strain engineering and geometric frustration as an on\u2010demand strategy for fabricating spontaneous rolling \u201corigami\u201d structures with programmable multistability across multiple length scales are exploited. Through experiments, theory, and finite element simulations, it is demonstrated that a strain\u2010engineered bilayer structure can make a transition from a monostable, doubly curved shape to a neutrally stable, developable configuration, depending on a dimensionless parameter that is determined through the plate's geometry and misfit strain. In addition, the doubly curved region near the edge can play a significant role in deciding the final bending direction of the strained bilayer due to edge effects. A strain\u2010engineering approach is further proposed to generate various 3D structures by programming the geometry, misfit strain, and mechanical properties of the bilayer units, for instance, a self\u2010folding buckyball structure. 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