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Despite the remarkable progress on sensors development, there are still some limitations, for instance, the requirement of high operating temperatures, and that most sensors are solely dedicated to individual gas monitoring. Herein, an ultrasensitive, highly discriminative platform is demonstrated for the detection and identification of ammonia and phosphine at room temperature using a graphene nanosensor. Graphene is exfoliated and successfully functionalized by copper phthalocyanine derivate. In combination with highly efficient machine learning techniques, the developed graphene nanosensor demonstrates an excellent gas identification performance even at ultralow concentrations: 100\u2009ppb NH\n                      <jats:sub>3<\/jats:sub>\n                      (accuracy\u2014100.0%, sensitivity\u2014100.0%, specificity\u2014100.0%) and 100\u2009ppb PH\n                      <jats:sub>3<\/jats:sub>\n                      (accuracy\u201477.8%, sensitivity\u201475.0%, and specificity\u201478.6%). Molecular dynamics simulation results reveal that the copper phthalocyanine derivate molecules attached to the graphene surface facilitate the adsorption of ammonia molecules owing to hydrogen bonding interactions. The developed smart gas sensing platform paves a path to design a highly selective, highly sensitive, miniaturized, low\u2010power consumption, nondedicated, smart gas sensing system toward a wide spectrum of gases.\n                    <\/jats:p>\n                  <\/jats:sec>","DOI":"10.1002\/aisy.202200016","type":"journal-article","created":{"date-parts":[[2022,3,19]],"date-time":"2022-03-19T07:56:10Z","timestamp":1647676570000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":67,"title":["Machine Learning\u2010Enabled Smart Gas Sensing Platform for Identification of Industrial Gases"],"prefix":"10.1002","volume":"4","author":[{"given":"Shirong","family":"Huang","sequence":"first","affiliation":[{"name":"Institute for Materials Science and Max Bergmann Center for Biomaterials TU Dresden  01062 Dresden Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Alexander","family":"Croy","sequence":"additional","affiliation":[{"name":"Institute for Physical Chemistry Friedrich Schiller University Jena  Helmholtzweg 4 07743 Jena Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Luis Antonio","family":"Panes-Ruiz","sequence":"additional","affiliation":[{"name":"Institute for Materials Science and Max Bergmann Center for Biomaterials TU Dresden  01062 Dresden Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Vyacheslav","family":"Khavrus","sequence":"additional","affiliation":[{"name":"SmartNanotubes Technologies GmbH  Dresdener Str. 172 01705 Freital Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Viktor","family":"Bezugly","sequence":"additional","affiliation":[{"name":"SmartNanotubes Technologies GmbH  Dresdener Str. 172 01705 Freital Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9899-1409","authenticated-orcid":false,"given":"Bergoi","family":"Ibarlucea","sequence":"additional","affiliation":[{"name":"Institute for Materials Science and Max Bergmann Center for Biomaterials TU Dresden  01062 Dresden Germany"},{"name":"Center for Advancing Electronics Dresden (CFAED) TU Dresden  01062 Dresden Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Gianaurelio","family":"Cuniberti","sequence":"additional","affiliation":[{"name":"Institute for Materials Science and Max Bergmann Center for Biomaterials TU Dresden  01062 Dresden Germany"},{"name":"Center for Advancing Electronics Dresden (CFAED) TU Dresden  01062 Dresden Germany"},{"name":"Dresden Center for Computational Materials Science (DCMS) TU Dresden  01062 Dresden Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2022,3,19]]},"reference":[{"key":"e_1_2_8_2_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.electacta.2018.11.215"},{"key":"e_1_2_8_3_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.talanta.2019.01.060"},{"key":"e_1_2_8_4_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.snb.2013.01.014"},{"key":"e_1_2_8_5_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.snb.2004.11.054"},{"key":"e_1_2_8_6_1","first-page":"1295","volume-title":"Hamilton & Hardy's Industrial Toxicology","author":"Perkins M. 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