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Herein, stretchable strain sensors capable of operating over multi\u2010strain range and having an excellent gauge factor are presented. The systematic study, carried out with different combinations of elastomer, conductive filler, and graphene\u2013carbon paste (GCP), revealed that the sensors exhibit excellent stretchability when only filler particles are present in the elastomer, and they exhibit high sensitivity when filler particles are mixed with GCP. The molecular dynamics simulations show that the addition of GCP to the elastomer\u2010filler composite helps to attain an excellent sensor response with wide range stretchability. Thus, sensors\u2019 response can be tuned by using selected material composition. Accordingly, the strain sensor with 50\u2009wt% GCP reveals 500% stretchability and a maximum gauge factor of 504. Likewise, 150\u2009wt% GCP loading lead to sensors with 45% stretchability and an unprecedented gauge factor of 1\u2009834\u2009140. The capability to detect the small\u2010 to large\u2010scale strains makes the presented sensors attractive for monitoring the movements of body parts\u2013which range from small movements during facial expression to large movement experienced by the limb joints.<\/jats:p><\/jats:sec>","DOI":"10.1002\/aisy.202200043","type":"journal-article","created":{"date-parts":[[2022,6,17]],"date-time":"2022-06-17T02:31:11Z","timestamp":1655433071000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":35,"title":["Ultra\u2010High Gauge Factor Strain Sensor with Wide\u2010Range Stretchability"],"prefix":"10.1002","volume":"4","author":[{"given":"Yogeenth","family":"Kumaresan","sequence":"first","affiliation":[{"name":"Bendable Electronics and Sensing Technologies (BEST) Group University of Glasgow  Glasgow G12 8QQ UK"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shashank","family":"Mishra","sequence":"additional","affiliation":[{"name":"Bendable Electronics and Sensing Technologies (BEST) Group University of Glasgow  Glasgow G12 8QQ UK"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Oliver","family":"Ozioko","sequence":"additional","affiliation":[{"name":"Bendable Electronics and Sensing Technologies (BEST) Group University of Glasgow  Glasgow G12 8QQ UK"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Radu","family":"Chirila","sequence":"additional","affiliation":[{"name":"Bendable Electronics and Sensing Technologies (BEST) Group University of Glasgow  Glasgow G12 8QQ UK"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3858-3841","authenticated-orcid":false,"given":"Ravinder","family":"Dahiya","sequence":"additional","affiliation":[{"name":"Bendable Electronics and Sensing Technologies (BEST) Group University of Glasgow  Glasgow G12 8QQ UK"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2022,6,16]]},"reference":[{"key":"e_1_2_9_2_1","doi-asserted-by":"publisher","DOI":"10.1109\/JPROC.2018.2890729"},{"key":"e_1_2_9_2_2","doi-asserted-by":"publisher","DOI":"10.1109\/JPROC.2019.2941665"},{"key":"e_1_2_9_3_1","doi-asserted-by":"publisher","DOI":"10.1002\/aisy.202100091"},{"key":"e_1_2_9_4_1","doi-asserted-by":"publisher","DOI":"10.1109\/JIOT.2020.3048282"},{"key":"e_1_2_9_4_2","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.1c12526"},{"key":"e_1_2_9_5_1","doi-asserted-by":"publisher","DOI":"10.1002\/aelm.202000445"},{"key":"e_1_2_9_6_1","doi-asserted-by":"publisher","DOI":"10.1002\/aisy.202100092"},{"key":"e_1_2_9_7_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.0c06435"},{"key":"e_1_2_9_7_2","doi-asserted-by":"publisher","DOI":"10.1038\/s41928-018-0071-7"},{"key":"e_1_2_9_7_3","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.1c14228"},{"key":"e_1_2_9_8_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsaelm.0c00278"},{"key":"e_1_2_9_8_2","doi-asserted-by":"publisher","DOI":"10.1109\/TED.2020.2982732"},{"key":"e_1_2_9_9_1","doi-asserted-by":"publisher","DOI":"10.1002\/admt.201700136"},{"key":"e_1_2_9_10_1","doi-asserted-by":"publisher","DOI":"10.1002\/aisy.201900165"},{"key":"e_1_2_9_11_1","doi-asserted-by":"publisher","DOI":"10.1002\/adom.201600451"},{"key":"e_1_2_9_12_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.pmatsci.2019.100617"},{"key":"e_1_2_9_12_2","doi-asserted-by":"publisher","DOI":"10.1002\/aisy.202000039"},{"key":"e_1_2_9_13_1","doi-asserted-by":"publisher","DOI":"10.1007\/978-94-007-0579-1"},{"key":"e_1_2_9_13_2","author":"Fu X.","year":"2019","journal-title":"J. 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