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Herein, the development of hybrid piezoelectric\u2013magnetic self\u2010sensing actuator (HPMSA) that can both sense and actuate is proposed. This iron oxide\/functionalized carbon nanotube\/polyvinylidene fluoride film optimizes both piezoelectric and magnetic properties through dual\u2010alignment fabrication, utilizing strong element bonds for simultaneous alignment. Magnetic nanoparticles are advantageous over nanorods due to latter's randomized shape anisotropy decreasing magnetization. The dual magnetic and mechanical processing increases polar <jats:italic>\u03b2<\/jats:italic>\u2010crystal content to 88%, where magnetic alignment alone increases degree of crystallinity to 66%. As a vibration damper, HPMSA operates within 40\u2013600\u2009Hz frequency, with a sensing sensitivity of 2.5\u2009mV\u2009g<jats:sup>\u22121<\/jats:sup> and 0.72\u2009m\u2009s<jats:sup>\u22122<\/jats:sup> weighted acceleration damping, lowering passenger health risks. 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