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Photoswitches\u2010based solar thermal materials could achieve super\u2010high photothermal conversion efficiency, while it remains a great challenge to apply such materials in biomedical treatments. Herein, a photothermal conversion film with good mechanical strength is designed through electrostatically complexing Ca\n                    <jats:sup>2+<\/jats:sup>\n                    \u2010cross\u2010linked alginate with azobenzene\u2010containing ammonium surfactant. The non\u2010covalent framework provides sufficient free volume for the trans\u2013cis isomerization of azobenzene in film state, and thereby this film gains merits of easy energy charging, energy density up to 481.0 J\/g, and controlled heat release by forming a closed system with efficient photothermal conversion. The film could on\u2010demand rise the environmental temperature at a range from room temperature to 75\u00b0C by regulating the film layers. This film exhibits characteristics of light weight, tailorability and good biocompatibility that are suitable for wound healing treatment. In animal studies, attractive wound healing promoting effect is achieved from the photothermal therapy with this film as dressing biomaterial, which is attributed to the created \u201chot spring\u201d condition for reducing inflammation and enhancing tissue remodeling. This study realizes the biomedical application of molecular solar thermal materials by combining the photoswitches\u2010based closed\u2010system and biomacromolecules\u2010based film together in a non\u2010covalent designing strategy.\n                  <\/jats:p>","DOI":"10.1002\/adhm.71860","type":"journal-article","created":{"date-parts":[[2026,10,15]],"date-time":"2026-10-15T15:23:51Z","timestamp":1792077831000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Easy Tailorable Alginate Film Gaining Super\u2010Efficient Photothermal Conversion From Closed\u2010System Design for Antibacterial and Wound Healing Applications"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-7991-0194","authenticated-orcid":false,"given":"Zhongtao","family":"Wu","sequence":"first","affiliation":[{"name":"Key Laboratory of Optic\u2010electric Sensing and Analytical Chemistry for Life Science, MOE; Shandong Key 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