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These compounds have shown remarkable optical features in addition to interesting electrical properties, and hence they are recognized as very suitable and versatile options for the development of functional materials. This progress report is focused on current and future use of CS structures and molecular assemblies with the aim of exploring and developing for the next generations of functional materials. A critical selection of illustrative materials that contain the CS motif, including relevant subfamilies such as the dicyanodistyrylbenzene and 2,3,3\u2010triphenylacrylonitrile shows how, driven by the self\u2010assembly of CS blocks, a variety of properties, effects, and possibilities for practical applications can be offered to the scientific community, through different rational routes for the elaboration of advanced materials. A survey is provided on the research efforts directed toward promoting the self\u2010assembly of the solid state (polycrystalline solids, thin films, and single crystals), liquid crystals, nanostructures, and gels with multistimuli responsiveness, and applications for sensors, organic light\u2010emitting diodes, organic field effect transistors, organic lasers, solar cells, or bioimaging purposes.<\/jats:p>","DOI":"10.1002\/adma.201704161","type":"journal-article","created":{"date-parts":[[2017,11,29]],"date-time":"2017-11-29T10:30:34Z","timestamp":1511951434000},"source":"Crossref","is-referenced-by-count":247,"title":["Self\u2010Assembled \u03b1\u2010Cyanostilbenes for Advanced Functional Materials"],"prefix":"10.1002","volume":"30","author":[{"given":"Marta","family":"Mart\u00ednez\u2010Abad\u00eda","sequence":"first","affiliation":[{"name":"Departamento de Qu\u00edmica Org\u00e1nica \u2013 Facultad de Ciencias Instituto de Ciencia de Materiales de Arag\u00f3n (ICMA) Universidad de Zaragoza \u2013 CSIC  50009 Zaragoza Spain"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Raquel","family":"Gim\u00e9nez","sequence":"additional","affiliation":[{"name":"Departamento de Qu\u00edmica Org\u00e1nica \u2013 Facultad de Ciencias Instituto de Ciencia de Materiales de Arag\u00f3n (ICMA) Universidad de Zaragoza \u2013 CSIC  50009 Zaragoza Spain"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4416-1036","authenticated-orcid":false,"given":"Mar\u00eda Blanca","family":"Ros","sequence":"additional","affiliation":[{"name":"Departamento de Qu\u00edmica Org\u00e1nica \u2013 Facultad de Ciencias Instituto de Ciencia de Materiales de Arag\u00f3n (ICMA) Universidad de Zaragoza \u2013 CSIC  50009 Zaragoza Spain"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2017,11,28]]},"reference":[{"key":"e_1_2_10_1_1","doi-asserted-by":"publisher","DOI":"10.1021\/cr050152i"},{"key":"e_1_2_10_1_2","doi-asserted-by":"publisher","DOI":"10.1021\/cr0501339"},{"key":"e_1_2_10_1_3","doi-asserted-by":"publisher","DOI":"10.1021\/cr900263j"},{"key":"e_1_2_10_1_4","doi-asserted-by":"publisher","DOI":"10.1039\/C0CS00058B"},{"key":"e_1_2_10_1_5","doi-asserted-by":"publisher","DOI":"10.1533\/9780857098764"},{"key":"e_1_2_10_1_6","doi-asserted-by":"publisher","DOI":"10.1002\/9783527653454"},{"key":"e_1_2_10_1_7","doi-asserted-by":"publisher","DOI":"10.1039\/C4CS00334A"},{"key":"e_1_2_10_2_1","volume-title":"Photophysics of Aromatic Molecules","author":"Birks J. 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