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The major challenge of this system is the polysulfide shuttle, which results in poor cycling efficiency. In this work, a highly N\u2010doped carbon\/graphene (NC\/G) sheet is designed as a sulfur host, which combines the merits of abundant N active sites and high electrical conductivity to achieve in situ anchoring\u2013conversion of lithium polysulfides (LiPSs). Such a host not only has strong binding with LiPSs but also promotes redox kinetics, which are revealed by both experimental investigations and theoretical studies. The sulfur cathode based on the NC\/G host exhibits a high initial capacity of 1380 mA h g<jats:sup>\u22121<\/jats:sup> and a superior cycle stability with a low capacity decay of 0.037% per cycle within 500 cycles at 2 C. Steady areal capacity with a high sulfur loading (5.6 mg cm<jats:sup>\u22122<\/jats:sup>) is also attained even without the addition of LiNO<jats:sub>3<\/jats:sub> in the electrolyte. This work proposes and illustrates the importance of in situ anchoring\u2013conversion of LiPSs, offering a new strategy to design multifunctional sulfur hosts for high\u2010performance Li\u2013S batteries.<\/jats:p>","DOI":"10.1002\/adma.201906357","type":"journal-article","created":{"date-parts":[[2019,12,27]],"date-time":"2019-12-27T02:57:13Z","timestamp":1577415433000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":139,"title":["Integrating Conductivity, Immobility, and Catalytic Ability into High\u2010N Carbon\/Graphene Sheets as an Effective Sulfur Host"],"prefix":"10.1002","volume":"32","author":[{"given":"Huifang","family":"Xu","sequence":"first","affiliation":[{"name":"School of Chemical Engineering and Light Industry Guangdong University of Technology  Guangzhou 510006 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