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However, record\u2010breaking devices have not shown compatibility with large\u2010scale production via solution processing in particular due to the use of halogenated environment\u2010threatening solvents. Here, slot\u2010die fabrication with processing involving hydrocarbon\u2010based solvents is used to realize highly efficient and environmentally friendly OSCs. Highly compatible slot\u2010die coating with roll\u2010to\u2010roll processing using halogenated (chlorobenzene (CB)) and hydrocarbon solvents (1,2,4\u2010trimethylbenzene (TMB) and\n                    <jats:italic>ortho<\/jats:italic>\n                    \u2010xylene (\n                    <jats:italic>o<\/jats:italic>\n                    \u2010XY)) is used to fabricate photoactive films. Controlled solution and substrate temperatures enable similar aggregation states in the solution and similar kinetics processes during film formation. The optimized blend film nanostructures for different solvents in the highly efficient PM6:Y6 blend is adopted to show a similar morphology, which results in device efficiencies of 15.2%, 15.4%, and 15.6% for CB, TMB, and o\u2010XY solvents. This approach is successfully extended to other donor\u2013acceptor combinations to demonstrate the excellent universality of this method. The results combine a method to optimize the aggregation state and film formation kinetics with the fabrication of OSCs with environmentally friendly solvents by slot\u2010die coating, which is a critical finding for the future development of OSCs in terms of their scalable production and high\u2010performance.\n                  <\/jats:p>","DOI":"10.1002\/adma.202002302","type":"journal-article","created":{"date-parts":[[2020,8,28]],"date-time":"2020-08-28T08:56:49Z","timestamp":1598605009000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":238,"title":["Hot Hydrocarbon\u2010Solvent Slot\u2010Die Coating Enables High\u2010Efficiency Organic Solar Cells with Temperature\u2010Dependent Aggregation Behavior"],"prefix":"10.1002","volume":"32","author":[{"given":"Heng","family":"Zhao","sequence":"first","affiliation":[{"name":"State Key Laboratory for Mechanical Behavior of Materials Xi'an Jiaotong University  Xi'an 710049 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