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Here, it is shown that uniform and continuous layers of copper can be intercalated within the van der Waals gap of bulk MoS\n                    <jats:sub>2<\/jats:sub>\n                    resulting in a unique Cu\u2013MoS\n                    <jats:sub>2<\/jats:sub>\n                    hybrid. The new Cu\u2013MoS\n                    <jats:sub>2<\/jats:sub>\n                    hybrid, which remains semiconducting, possesses a unique plasmon resonance at an energy of \u22481eV, giving rise to enhanced optoelectronic activity. Compared with high\u2010performance MoS\n                    <jats:sub>2<\/jats:sub>\n                    photodetectors, copper\u2010enhanced devices are superior in their spectral response, which extends into the infrared, and also in their total responsivity, which exceeds 10\n                    <jats:sup>4<\/jats:sup>\n                    A W\n                    <jats:sup>\u22121<\/jats:sup>\n                    . 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