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Here, an ultrasensitive self\u2010powered mechanoluminescence smart skin (SPMSS) inspired by the luminescence mechanism of cephalopod skin and the ultrasensitive response of spider\u2010slit\u2010organ is developed. Benefitting from the unique strain\u2010dependent microcrack structure design based on Ti\n                    <jats:sub>3<\/jats:sub>\n                    C\n                    <jats:sub>2<\/jats:sub>\n                    T\n                    <jats:italic>\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    (MXene)\/carbon nanotube synergistic interaction, SPMSS possesses excellent strain sensing performances including ultralow detection limit (0.001% strain), ultrahigh sensitivity (gauge factor, GF = 3.92 \u00d7 10\n                    <jats:sup>7<\/jats:sup>\n                    ), ultrafast response time (5\u00a0ms), and superior durability and stability (&gt;45\u2009000 cycles). Synchronously, SPMSS exhibits tunable and highly sensitive mechanoluminescence (ML) features under stretching. A relationship between ML features, strain sensing performances, and the deformation has been established successfully. Importantly, the SPMSS demonstrates excellent properties as triboelectric nanogenerator (4 \u00d7 4 cm\n                    <jats:sup>2<\/jats:sup>\n                    ), including ultrahigh triboelectric output (open\u2010circuit voltage\n                    <jats:italic>V<\/jats:italic>\n                    <jats:sub>OC<\/jats:sub>\n                    \u00a0= 540\u00a0V, short\u2010circuit current\n                    <jats:italic>I<\/jats:italic>\n                    <jats:sub>SC<\/jats:sub>\n                    \u00a0= 42 \u00b5A, short\u2010circuit charge\n                    <jats:italic>Q<\/jats:italic>\n                    <jats:sub>SC<\/jats:sub>\n                    \u00a0= 317 nC) and power density (7.42 W m\n                    <jats:sup>\u22122<\/jats:sup>\n                    ), endowing the smart skin with reliable power source supply and self\u2010powered sensing ability. This bioinspired smart skin exhibits multifunctional applications in health monitoring, visual sensing, and self\u2010powered sensing, showing great potential in artificial intelligence.\n                  <\/jats:p>","DOI":"10.1002\/adma.202102332","type":"journal-article","created":{"date-parts":[[2021,9,23]],"date-time":"2021-09-23T14:01:25Z","timestamp":1632405685000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":247,"title":["Bioinspired Multifunctional Photonic\u2010Electronic Smart Skin for Ultrasensitive Health Monitoring, for Visual and Self\u2010Powered Sensing"],"prefix":"10.1002","volume":"33","author":[{"given":"Yi","family":"Zhao","sequence":"first","affiliation":[{"name":"School of Materials Science and Engineering Key Laboratory of Materials Processing and Mold Ministry of Education Zhengzhou University  Zhengzhou 450001 P. R. 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