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In these compounds, spin\u2013phonon coupling (SPC) typically plays a crucial role in magnetic fluctuations, magnon dissipation, and ultimately establishing long\u2010range ferromagnetic order. However, a systematic understanding of SPC in 2D magnets that combines theory and experiment is still lacking. In this work, monolayer chromium tribromide is studied to investigate SPC in 2D magnets via Raman spectroscopy and first principle calculations. The experimental Curie temperature and phonon shifts are found to be in good agreement with the numerical simulations. Specifically, it is demonstrated how magnetic exchange interactions affect phonon vibrations, which helps establish design fundamentals for 2D magnetic materials and other related devices.<\/jats:p>","DOI":"10.1002\/adma.202108506","type":"journal-article","created":{"date-parts":[[2022,3,14]],"date-time":"2022-03-14T05:09:03Z","timestamp":1647234543000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":23,"title":["Spin\u2013Phonon Coupling in Ferromagnetic Monolayer Chromium Tribromide"],"prefix":"10.1002","volume":"34","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-8751-7082","authenticated-orcid":false,"given":"Jiangbin","family":"Wu","sequence":"first","affiliation":[{"name":"Ming Hsieh Department of Electrical and Computer Engineering University of Southern California  Los Angeles CA 90089 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