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The correlated rattling of Na atoms in the zigzag chains and the origin of the low thermal conductivity is uncovered via experimental and computational analyses. The Na atoms behave as oscillators along the tunnel, resulting in substantial interactions between Na atoms in the chain and between the chain and framework. In these intermetallic compounds, a shorter inter\u2010rattler distance results in lower thermal conductivity, suggesting that phonon scattering by the correlated rattling Na\u2010chains is enhanced. These results provide new insights into the behavior of thermoelectric materials with low thermal conductivity and suggest strategies for the development of such materials that utilize the correlated rattling.<\/jats:p>","DOI":"10.1002\/adma.202207646","type":"journal-article","created":{"date-parts":[[2022,12,17]],"date-time":"2022-12-17T05:54:28Z","timestamp":1671256468000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":25,"title":["Correlated Rattling of Sodium\u2010Chains Suppressing Thermal Conduction in Thermoelectric Stannides"],"prefix":"10.1002","volume":"35","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-0996-0975","authenticated-orcid":false,"given":"Takahiro","family":"Yamada","sequence":"first","affiliation":[{"name":"Institute of Multidisciplinary Research for Advanced Material Tohoku University  2\u20101\u20101 Katahira, Aoba\u2010ku Sendai 980\u20108577 Japan"},{"name":"PRESTO Japan Science and Technology Agency  4\u20101\u20108 Honcho Kawaguchi 332\u20100012 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2029-2525","authenticated-orcid":false,"given":"Masato","family":"Yoshiya","sequence":"additional","affiliation":[{"name":"Division of Materials and Manufacturing Science Graduate School of Engineering Osaka University  2\u20101 Yamadaoka Suita Osaka 565\u20100871 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Masahiro","family":"Kanno","sequence":"additional","affiliation":[{"name":"Institute of Multidisciplinary Research for Advanced Material Tohoku University  2\u20101\u20101 Katahira, Aoba\u2010ku Sendai 980\u20108577 Japan"},{"name":"Department of Metallurgy Materials Science and Materials Processing Graduate School of Engineering Tohoku University  6\u20106\u201004 Aramaki Aza Aoba, Aoba\u2010ku Sendai 980\u20108579 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5792-0113","authenticated-orcid":false,"given":"Hiroshi","family":"Takatsu","sequence":"additional","affiliation":[{"name":"Graduate School of Engineering Kyoto University  Nishikyo\u2010ku Kyoto 615\u20108510 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7992-5636","authenticated-orcid":false,"given":"Takuji","family":"Ikeda","sequence":"additional","affiliation":[{"name":"Research Institute for Chemical Process Technology National Institute of Advanced Industrial Science and Technology (AIST Tohoku)  4\u20102\u20101 Nigatake, Miyagino\u2010ku Sendai 983\u20108551 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4005-169X","authenticated-orcid":false,"given":"Hideaki","family":"Nagai","sequence":"additional","affiliation":[{"name":"Research Institute for Energy Conservation National Institute of Advanced Industrial Science and Technology (AIST)  1\u20101\u20101 Higashi Tsukuba Ibaraki 305\u20108565 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-7931-5210","authenticated-orcid":false,"given":"Hisanori","family":"Yamane","sequence":"additional","affiliation":[{"name":"Institute of Multidisciplinary Research for Advanced Material Tohoku University  2\u20101\u20101 Katahira, Aoba\u2010ku Sendai 980\u20108577 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3911-9864","authenticated-orcid":false,"given":"Hiroshi","family":"Kageyama","sequence":"additional","affiliation":[{"name":"Graduate School of Engineering Kyoto University  Nishikyo\u2010ku Kyoto 615\u20108510 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2023,1,26]]},"reference":[{"key":"e_1_2_8_1_1","doi-asserted-by":"publisher","DOI":"10.1201\/9781420049718"},{"key":"e_1_2_8_2_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.aak9997"},{"key":"e_1_2_8_3_1","doi-asserted-by":"publisher","DOI":"10.1038\/181834a0"},{"key":"e_1_2_8_4_1","doi-asserted-by":"publisher","DOI":"10.1039\/c3cp52942h"},{"key":"e_1_2_8_5_1","doi-asserted-by":"publisher","DOI":"10.1038\/nature11439"},{"key":"e_1_2_8_6_1","doi-asserted-by":"publisher","DOI":"10.1088\/0034-4885\/51\/4\/001"},{"key":"e_1_2_8_7_1","first-page":"407","volume-title":"CRC Handbook of Thermoelectrics","author":"Slack G. 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