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Here, a generic van der Waals epitaxial approach is developed to synthesize the 2D ternary chromium tellurium compounds with thicknesses down to mono\u2010, bi\u2010, tri\u2010, and few\u2010unit cells\u00a0(UC). The Mn\n                    <jats:sub>0.14<\/jats:sub>\n                    Cr\n                    <jats:sub>0.86<\/jats:sub>\n                    Te evolves from intrinsic ferromagnetic behavior in bi\u2010UC, tri\u2010UC, and few\u2010UC to temperature\u2010induced ferrimagnetic behavior as the thickness increases, resulting in a sign reversal of the anomalous Hall resistance. Temperature\u2010 and thickness\u2010tunable labyrinthine\u2010domain ferromagnetic behaviors are derived from the dipolar interactions in Fe\n                    <jats:sub>0.26<\/jats:sub>\n                    Cr\n                    <jats:sub>0.74<\/jats:sub>\n                    Te and Co\n                    <jats:sub>0.40<\/jats:sub>\n                    Cr\n                    <jats:sub>0.60<\/jats:sub>\n                    Te. Furthermore, the dipolar\u2010interaction\u2010induced stripe domain and field\u2010induced domain wall (DW) motion velocity are studied, and multibit data storage is realized through an abundant DW state. The magnetic storage can function in neuromorphic computing tasks, and the pattern recognition accuracy can reach up to 97.93%, which is similar to the recognition accuracy of ideal software\u2010based training (98.28%). Room\u2010temperature ferromagnetic chromium tellurium compounds with intriguing spin configurations can significantly promote the exploration of the processing, sensing, and storage based on 2D magnetic systems.\n                  <\/jats:p>","DOI":"10.1002\/adma.202209346","type":"journal-article","created":{"date-parts":[[2023,3,2]],"date-time":"2023-03-02T16:29:06Z","timestamp":1677774546000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":14,"title":["Room\u2010Temperature Intrinsic Ferromagnetic Chromium Tellurium Compounds with Thickness\u2010Tunable Magnetic Texture"],"prefix":"10.1002","volume":"35","author":[{"given":"Yao","family":"Wen","sequence":"first","affiliation":[{"name":"Key Laboratory of Artificial Micro\u2010 and Nano\u2010structures of Ministry of Education School of Physics and Technology Wuhan University  Wuhan 430072 P. R. 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