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Perovskite (FAPbI\n                    <jats:sub>3<\/jats:sub>\n                    ) films based on one\u2010step antisolvent methods usually suffer from chaotic orientations due to the inevitable intermediate phase conversion from intermediates of PbI\n                    <jats:sub>2<\/jats:sub>\n                    \u2022DMSO, FA\n                    <jats:sub>2<\/jats:sub>\n                    Pb\n                    <jats:sub>3<\/jats:sub>\n                    I\n                    <jats:sub>8<\/jats:sub>\n                    \u20224DMSO, and\n                    <jats:italic>\u03b4<\/jats:italic>\n                    \u2010FAPbI\n                    <jats:sub>3<\/jats:sub>\n                    to\n                    <jats:italic>\u03b1<\/jats:italic>\n                    \u2010FAPbI\n                    <jats:sub>3<\/jats:sub>\n                    . Here, a high\u2010quality perovskite film with (111) preferred orientation ((111)\u2010\n                    <jats:italic>\u03b1<\/jats:italic>\n                    \u2010FAPbI\n                    <jats:sub>3<\/jats:sub>\n                    ) using a short\u2010chain isomeric alcohol antisolvent, isopropanol (IPA) or isobutanol (IBA), is reported. The interaction between IPA and PbI\n                    <jats:sub>2<\/jats:sub>\n                    leads to a corner\u2010sharing structure instead of an edge\u2010sharing PbI\n                    <jats:sub>2<\/jats:sub>\n                    octahedron, sidestepping the formation of these intermediates. With the volatilization of IPA, FA\n                    <jats:sup>+<\/jats:sup>\n                    can replace IPA in situ to form\n                    <jats:italic>\u03b1<\/jats:italic>\n                    \u2010FAPbI\n                    <jats:sub>3<\/jats:sub>\n                    along the (111) direction. Compared to randomly orientated perovskites, the dominantly (111) orientated perovskite ((111)\u2010perovskite) exhibits improved carrier mobility, uniform surface potential, suppressed film defects and enhanced photostability. PSCs based on the (111)\u2010perovskite films show 22% power conversion efficiency and excellent stability, which remains unchanged after 600\u00a0h continuous working at maximum power point, and 95% after 2000\u00a0h of storage in atmosphere environment.\n                  <\/jats:p>","DOI":"10.1002\/adma.202301115","type":"journal-article","created":{"date-parts":[[2023,4,7]],"date-time":"2023-04-07T02:24:50Z","timestamp":1680834290000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":79,"title":["(111)\u2010Dominated Perovskite Films by Antisolvent Engineering"],"prefix":"10.1002","volume":"35","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-5267-3157","authenticated-orcid":false,"given":"Xiangyu","family":"Sun","sequence":"first","affiliation":[{"name":"Beijing Key Laboratory of Construction\u2010Tailorable Advanced Functional Materials and Green Applications Experimental Center of Advanced Materials School of Materials 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