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Achieving high strength and large deformation simultaneously is a huge challenge. Herein, high\u2010strength ionogels are developed through the synergy of force\u2010induced crystallization and halometallate ionic liquid created supramolecular ionic networks. The prepared poly(vinyl alcohol)\/halometallate ionic liquid ionogels show excellent mechanical properties, including ultimate fracture stress (63.1\u00a0\u00b1\u00a02.1\u00a0MPa), strain (5248\u00a0\u00b1\u00a0113%), and unprecedented toughness (1947\u00a0\u00b1\u00a052\u00a0MJ\u00a0m\n                    <jats:sup>\u22123<\/jats:sup>\n                    ), which is much higher than that of most metals and alloys. Furthermore, the ionogels can achieve reversibility by water to realize green recovery and restoration of damaged mechanical properties.\n                  <\/jats:p>","DOI":"10.1002\/adma.202301383","type":"journal-article","created":{"date-parts":[[2023,4,24]],"date-time":"2023-04-24T16:34:45Z","timestamp":1682354085000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":171,"title":["Supramolecular Ionogels Tougher than Metals"],"prefix":"10.1002","volume":"35","author":[{"given":"Weizheng","family":"Li","sequence":"first","affiliation":[{"name":"Jiangsu Engineering Laboratory of Novel Functional Polymeric Materials Jiangsu Key Laboratory of Advanced Negative Carbon Technologies College of Chemistry Suzhou Key Laboratory of Soft Material and New Energy College of Chemistry Chemical Engineering and Materials Science Soochow University  Suzhou 215123 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