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The typical polarization rotation of transmitted light is usually wavelength dependent, namely the optical rotatory dispersion. However, its dynamic tunability and intriguing collaboration with other optical degrees of freedom, especially the highly desired spatial phase, remain elusive. Herein, a bi\u2010chiral liquid crystalline nanostructure is proposed to induce an effect called reflective optical rotatory dispersion. Thanks to the independent manipulation of opposite\u2010handed self\u2010assembled helices, spin\u2010decoupled geometric phases are induced simultaneously. These naturally unite multi\u2010dimensions of light and versatile stimuli\u2010responsiveness of soft matter. Dynamic holography driven by heat and electric field is demonstrated with a fast response. For polychromatic light, the hybrid multiplexed holographic painting is exhibited with fruitful tunable colors. This study extends the ingenious construction of soft chiral superstructures, presents an open\u2010ended strategy for on\u2010demand light control, and enlightens advanced applications of display, optical computing, and communication.<\/jats:p>","DOI":"10.1002\/adma.202301714","type":"journal-article","created":{"date-parts":[[2023,5,10]],"date-time":"2023-05-10T15:09:16Z","timestamp":1683731356000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":70,"title":["Bi\u2010Chiral Nanostructures Featuring Dynamic Optical Rotatory Dispersion for Polychromatic Light Multiplexing"],"prefix":"10.1002","volume":"35","author":[{"given":"Si\u2010Jia","family":"Liu","sequence":"first","affiliation":[{"name":"National Laboratory of Solid State Microstructures Key Laboratory of Intelligent Optical Sensing and Manipulation College of Engineering and Applied Sciences, and Collaborative Innovation Center of Advanced Microstructures Nanjing 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