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Versatile fabrication and additive manufacturing methods are developed, but the ability to design a material for a given application is still limited. Here,\u00a0a novel strategy that enables target\u2010oriented manufacturing of ultra\u2010lightweight aerogels with on\u2010demand characteristics is introduced. The process relies on controllable liquid templating through interfacial complexation to generate tunable, stimuli\u2010responsive 3D\u2010structured (multiphase) filamentous liquid templates. The methodology involves nanoscale chemistry and microscale assembly of nanoparticles (NPs) at liquid\u2013liquid interfaces to produce hierarchical macroscopic aerogels featuring multiscale porosity, ultralow density (3.05\u20133.41\u00a0mg cm<jats:sup>\u22123<\/jats:sup>), and high compressibility (90%) combined with elastic resilience and instant shape recovery. The challenges are overcome facing ultra\u2010lightweight aerogels, including poor mechanical integrity and the inability to form predefined 3D constructs with on\u2010demand functionality, for a multitude of applications. The controllable nature of the coined methodology enables tunable electromagnetic interference shielding with high specific shielding effectiveness (39 893\u00a0dB cm<jats:sup>2<\/jats:sup> g<jats:sup>\u22121<\/jats:sup>), and one of the highest\u2010ever reported oil\u2010absorption capacities (487 times the initial weight of aerogel for chloroform), to be obtained. These properties originate from the engineerable nature of liquid templating, pushing the boundaries of lightweight materials to systematic function design and applications.<\/jats:p>","DOI":"10.1002\/adma.202302826","type":"journal-article","created":{"date-parts":[[2023,8,10]],"date-time":"2023-08-10T19:09:15Z","timestamp":1691694555000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":41,"title":["Liquid\u2010Templating Aerogels"],"prefix":"10.1002","volume":"35","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-4713-6883","authenticated-orcid":false,"given":"Seyyed Alireza","family":"Hashemi","sequence":"first","affiliation":[{"name":"Nanomaterials and Polymer Nanocomposites Laboratory School of Engineering University of British Columbia  Kelowna BC V1V 1V7 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ahmadreza","family":"Ghaffarkhah","sequence":"additional","affiliation":[{"name":"Nanomaterials and Polymer Nanocomposites Laboratory School of Engineering University of British Columbia  Kelowna BC V1V 1V7 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Milad","family":"Goodarzi","sequence":"additional","affiliation":[{"name":"Nanomaterials and Polymer Nanocomposites Laboratory School of Engineering University of British Columbia  Kelowna BC V1V 1V7 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Amir","family":"Nazemi","sequence":"additional","affiliation":[{"name":"Composites Research Network\u2010Okanagan Laboratory School of Engineering University of British Columbia Okanagan Campus  Kelowna BC V1V 1V7 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Gabriel","family":"Banvillet","sequence":"additional","affiliation":[{"name":"Bioproducts Institute Department of Chemical &amp; Biological Engineering Department of Chemistry and Department of Wood Science 2360 East Mall The University of British Columbia  Vancouver BC V6T 1Z3 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Abbas S.","family":"Milani","sequence":"additional","affiliation":[{"name":"Composites Research Network\u2010Okanagan Laboratory School of Engineering University of British Columbia Okanagan Campus  Kelowna BC V1V 1V7 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Masoud","family":"Soroush","sequence":"additional","affiliation":[{"name":"Department of Chemical and Biological Engineering Drexel University  Philadelphia PA 19104 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Orlando J.","family":"Rojas","sequence":"additional","affiliation":[{"name":"Bioproducts Institute Department of Chemical &amp; Biological Engineering Department of Chemistry and Department of Wood Science 2360 East Mall The University of British Columbia  Vancouver BC V6T 1Z3 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Seeram","family":"Ramakrishna","sequence":"additional","affiliation":[{"name":"Department of Mechanical Engineering Center for Nanofibers and Nanotechnology National University of Singapore  21 Lower Kent Ridge Road Singapore 119077 Singapore"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Stefan","family":"Wuttke","sequence":"additional","affiliation":[{"name":"Basque Centre for Materials Applications &amp; Nanostructures (BCMaterials) Bld. Martina Casiano  3rd. Floor UPV\/EHU Science Park Barrio Sarriena s\/n Leioa 48940 Spain"},{"name":"IKERBASQUE Basque Foundation for Science  Bilbao 48013 Spain"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Thomas P.","family":"Russell","sequence":"additional","affiliation":[{"name":"Polymer Science and Engineering Department University of Massachusetts Amherst  120 Governors Drive Amherst MA 01003 USA"},{"name":"Materials Sciences Division Lawrence Berkeley National Laboratory  1 Cyclotron Road Berkeley CA 94720 USA"},{"name":"Advanced Institute for Materials Research (WPI\u2010AIMR) Tohoku University  2\u20101\u20101 Katahira Aoba Sendai 980\u20138577 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Milad","family":"Kamkar","sequence":"additional","affiliation":[{"name":"Multi\u2010scale Materials Design Center Department of Chemical Engineering Waterloo Institute for Nanotechnology University of Waterloo  200 University Avenue West Waterloo Ontario N2L 3G1 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8812-5638","authenticated-orcid":false,"given":"Mohammad","family":"Arjmand","sequence":"additional","affiliation":[{"name":"Nanomaterials and Polymer Nanocomposites Laboratory School of Engineering University of British Columbia  Kelowna BC V1V 1V7 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2023,9,4]]},"reference":[{"key":"e_1_2_7_1_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.0c00577"},{"key":"e_1_2_7_1_2","doi-asserted-by":"publisher","DOI":"10.1021\/acsnano.2c00619"},{"key":"e_1_2_7_1_3","doi-asserted-by":"publisher","DOI":"10.1038\/nnano.2017.182"},{"key":"e_1_2_7_2_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.201800714"},{"key":"e_1_2_7_2_2","doi-asserted-by":"publisher","DOI":"10.1002\/adma.201806370"},{"key":"e_1_2_7_2_3","doi-asserted-by":"publisher","DOI":"10.1002\/anie.201908402"},{"key":"e_1_2_7_2_4","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemrev.0c01333"},{"key":"e_1_2_7_3_1","doi-asserted-by":"publisher","DOI":"10.1021\/jacs.1c00429"},{"key":"e_1_2_7_3_2","doi-asserted-by":"publisher","DOI":"10.1021\/jacs.0c02555"},{"key":"e_1_2_7_3_3","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202111252"},{"key":"e_1_2_7_3_4","doi-asserted-by":"publisher","DOI":"10.1021\/acssuschemeng.9b06099"},{"key":"e_1_2_7_4_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202016217"},{"key":"e_1_2_7_5_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-019-09042-y"},{"key":"e_1_2_7_5_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.chempr.2019.07.016"},{"key":"e_1_2_7_5_3","doi-asserted-by":"publisher","DOI":"10.1021\/acs.langmuir.8b00053"},{"key":"e_1_2_7_6_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.aaw8719"},{"key":"e_1_2_7_6_2","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202105500"},{"key":"e_1_2_7_7_1","volume-title":"Microfluidics: Modeling, Mechanics, and Mathematics","author":"Rapp B. 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