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The overuse of N\u2010containing fertilizers induces the increase of nitrate level in surface and ground waters, and substantial emission of nitrogen oxides causes heavy air pollution. Nitrogen gas, as the main component of air, has been used for mass ammonia production for over a century, providing enough nutrition for agriculture to support world population increase. In the last decade, researchers have made great efforts to develop ammonia processes under ambient conditions to combat the intensive energy consumption and high carbon emission associated with the Haber\u2013Bosch process. Among different techniques, electrochemical nitrate reduction reaction (NO\n                    <jats:sub>3<\/jats:sub>\n                    RR) can achieve nitrate removal and ammonia generation simultaneously using renewable electricity as the power, and there is an exponential growth of studies in this research direction. Here, a timely and comprehensive review on the important progresses of electrochemical NO\n                    <jats:sub>3<\/jats:sub>\n                    RR, covering the rational design of electrocatalysts, emerging C\uf8ffN coupling reactions, and advanced energy conversion and storage systems is provided. Moreover, future perspectives are proposed to accelerate the industrialized NH\n                    <jats:sub>3<\/jats:sub>\n                    production and green synthesis of chemicals, leading to a sustainable nitrogen cycle via prosperous N\u2010based electrochemistry.\n                  <\/jats:p>","DOI":"10.1002\/adma.202304021","type":"journal-article","created":{"date-parts":[[2023,6,9]],"date-time":"2023-06-09T08:37:24Z","timestamp":1686299844000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":699,"title":["Electrochemical Nitrate Reduction: Ammonia Synthesis and the Beyond"],"prefix":"10.1002","volume":"36","author":[{"given":"Yuecheng","family":"Xiong","sequence":"first","affiliation":[{"name":"Department of Chemistry City University of Hong Kong Kowloon Hong Kong SAR 999077 P. R. 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