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However, the practical control of the SDE necessities the precise tuning of current, temperature, magnetic field, or magnetism. Therefore, the mechanisms of the SDE must be understood to develop novel materials and devices capable of realizing the SDE under more controlled and robust conditions. This study demonstrates an intrinsic zero\u2010field SDE with an efficiency of up to 40% in Fe\/Pt\u2010inserted non\u2010centrosymmetric Nb\/V\/Ta superconducting artificial superlattices. The polarity and magnitude of the zero\u2010field SDE are controllable by the direction of magnetization, indicating that the effective exchange field acts on Cooper pairs. Furthermore, the first\u2010principles calculation indicates that the SDE can be enhanced by an asymmetric configuration of proximity induced magnetic moments in superconducting layers, which induces a magnetic toroidal moment. This study has important implications regarding the development of novel materials and devices that can effectively control the SDE. Moreover, the magnetization control of the SDE is expected to aid in the designing of superconducting quantum devices and establishing a material platform for topological superconductors.<\/jats:p>","DOI":"10.1002\/adma.202304083","type":"journal-article","created":{"date-parts":[[2023,7,6]],"date-time":"2023-07-06T11:02:39Z","timestamp":1688641359000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":25,"title":["Magnetization Control of Zero\u2010Field Intrinsic Superconducting Diode Effect"],"prefix":"10.1002","volume":"35","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-0319-7318","authenticated-orcid":false,"given":"Hideki","family":"Narita","sequence":"first","affiliation":[{"name":"Institute for Chemical Research Kyoto University  Gokasho Uji Kyoto 611\u20100011 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7565-7451","authenticated-orcid":false,"given":"Jun","family":"Ishizuka","sequence":"additional","affiliation":[{"name":"Faculty of Engineering Niigata University  Ikarashi Niigata 950\u20102181 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-7505-0059","authenticated-orcid":false,"given":"Daisuke","family":"Kan","sequence":"additional","affiliation":[{"name":"Institute for Chemical Research Kyoto University  Gokasho Uji Kyoto 611\u20100011 Japan"},{"name":"Center for Spintronics Research Network Institute for Chemical Research Kyoto University  Uji Kyoto 611\u20100011 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-1019-2512","authenticated-orcid":false,"given":"Yuichi","family":"Shimakawa","sequence":"additional","affiliation":[{"name":"Institute for Chemical Research Kyoto University  Gokasho Uji Kyoto 611\u20100011 Japan"},{"name":"Center for Spintronics Research Network Institute for Chemical Research Kyoto University  Uji Kyoto 611\u20100011 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Youichi","family":"Yanase","sequence":"additional","affiliation":[{"name":"Department of Physics Graduate School of Science Kyoto University  Kyoto 606\u20108502 Japan"},{"name":"Institute for Molecular Science  Okazaki 444\u20100867 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9629-0633","authenticated-orcid":false,"given":"Teruo","family":"Ono","sequence":"additional","affiliation":[{"name":"Institute for Chemical Research Kyoto University  Gokasho Uji Kyoto 611\u20100011 Japan"},{"name":"Center for Spintronics Research Network Institute for Chemical Research Kyoto University  Uji Kyoto 611\u20100011 Japan"},{"name":"Center for Spintronics Research Network Graduate School of Engineering Science Osaka University  Toyonaka 560\u20100043 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2023,8]]},"reference":[{"key":"e_1_2_8_1_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.87.236602"},{"key":"e_1_2_8_2_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.75.2004"},{"key":"e_1_2_8_3_1","doi-asserted-by":"publisher","DOI":"10.1088\/0953-8984\/8\/3\/012"},{"key":"e_1_2_8_4_1","doi-asserted-by":"publisher","DOI":"10.1126\/sciadv.1602390"},{"key":"e_1_2_8_5_1","doi-asserted-by":"publisher","DOI":"10.1063\/1.1789231"},{"key":"e_1_2_8_6_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41586-020-2590-4"},{"key":"e_1_2_8_7_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41586-022-04504-8"},{"key":"e_1_2_8_8_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41563-022-01300-7"},{"key":"e_1_2_8_9_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41565-021-01009-9"},{"key":"e_1_2_8_10_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-022-31954-5"},{"key":"e_1_2_8_11_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41565-022-01159-4"},{"key":"e_1_2_8_12_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41567-022-01700-1"},{"key":"e_1_2_8_13_1","doi-asserted-by":"publisher","DOI":"10.1063\/5.0109753"},{"key":"e_1_2_8_14_1","doi-asserted-by":"crossref","unstructured":"Y.Hou F.Nichele H.Chi A.Lodesani Y.Wu M. 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