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However, the long\u2010term viability of these hydrogel coatings is hindered by concerns regarding fatigue crack propagation and\/or delamination caused by repetitive volumetric expansion\/shrinkage during long\u2010term electrical interfacing. This study reports a general yet reliable approach to achieving a fatigue\u2010resistant conducting polymer hydrogel coating on conventional metallic bioelectrodes by engineering nanocrystalline domains at the interface between the hydrogel and metallic substrates. It demonstrates the efficacy of this robust, biocompatible, and fatigue\u2010resistant conducting hydrogel coating in cardiac pacing, showcasing its ability to effectively reduce the pacing threshold voltage and enhance the long\u2010term reliability of electric stimulation. This study findings highlight the potential of its approach as a promising design and fabrication strategy for the next generation of seamless bioelectronic\u00a0interfaces.<\/jats:p>","DOI":"10.1002\/adma.202304095","type":"journal-article","created":{"date-parts":[[2023,6,29]],"date-time":"2023-06-29T01:38:29Z","timestamp":1688002709000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":128,"title":["Mechanically\u2010Compliant Bioelectronic Interfaces through Fatigue\u2010Resistant Conducting Polymer Hydrogel Coating"],"prefix":"10.1002","volume":"35","author":[{"given":"Yu","family":"Xue","sequence":"first","affiliation":[{"name":"Department of Mechanical and Energy Engineering Southern University of Science and Technology  Shenzhen 518055 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xingmei","family":"Chen","sequence":"additional","affiliation":[{"name":"Department of Mechanical and Energy Engineering Southern University of Science and Technology  Shenzhen 518055 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Fucheng","family":"Wang","sequence":"additional","affiliation":[{"name":"Department of Mechanical and Energy Engineering Southern University of Science and Technology  Shenzhen 518055 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jingsen","family":"Lin","sequence":"additional","affiliation":[{"name":"Department of Mechanical and Energy Engineering Southern University of Science and Technology  Shenzhen 518055 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7171-405X","authenticated-orcid":false,"given":"Ji","family":"Liu","sequence":"additional","affiliation":[{"name":"Department of Mechanical and Energy Engineering Southern University of Science and Technology  Shenzhen 518055 China"},{"name":"Shenzhen Key Laboratory of Biomimetic Robotics and Intelligent Systems Department of Mechanical and Energy Engineering Southern University of Science and Technology  Shenzhen 518055 China"},{"name":"Shenzhen Key Laboratory of Intelligent Robotics and Flexible Manufacturing Systems Southern University of Science and Technology  Shenzhen 518055 China"},{"name":"Guangdong Provincial Key Laboratory of Human\u2010Augmentation and Rehabilitation Robotics in Universities Southern University of Science and Technology  Shenzhen 518055 China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2023,8,2]]},"reference":[{"key":"e_1_2_8_1_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41928-018-0024-1"},{"key":"e_1_2_8_2_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41587-019-0198-8"},{"key":"e_1_2_8_3_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.mattod.2019.12.026"},{"key":"e_1_2_8_4_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41563-020-0679-7"},{"key":"e_1_2_8_5_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.aaw9295"},{"key":"e_1_2_8_6_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41551-018-0335-6"},{"key":"e_1_2_8_7_1","doi-asserted-by":"publisher","DOI":"10.1126\/sciadv.aaw1066"},{"key":"e_1_2_8_8_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.201905522"},{"key":"e_1_2_8_9_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41928-018-0071-7"},{"key":"e_1_2_8_10_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.accounts.7b00548"},{"key":"e_1_2_8_11_1","doi-asserted-by":"publisher","DOI":"10.1126\/scitranslmed.aaw5858"},{"key":"e_1_2_8_12_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41551-017-0154-1"},{"key":"e_1_2_8_13_1","doi-asserted-by":"publisher","DOI":"10.1002\/mabi.201800112"},{"key":"e_1_2_8_14_1","first-page":"1","volume":"3","author":"Lind G.","year":"2013","journal-title":"Sci. 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