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Moreover, SCC can be tuned with the number of layers, electric field, or strain. Here, SCC in epitaxially grown 2D PtSe\n                    <jats:sub>2<\/jats:sub>\n                    by THz spintronic emission is studied since its 1T crystal symmetry and strong SOC favor SCC. High quality of as\u2010grown PtSe\n                    <jats:sub>2<\/jats:sub>\n                    layers is demonstrated, followed by in situ ferromagnet deposition by sputtering that leaves the PtSe\n                    <jats:sub>2<\/jats:sub>\n                    unaffected, resulting in well\u2010defined clean interfaces as evidenced with extensive characterization. Through this atomic growth control and using THz spintronic emission, the unique thickness\u2010dependent electronic structure of PtSe\n                    <jats:sub>2<\/jats:sub>\n                    allows the control of SCC. Indeed, the transition from the inverse Rashba\u2013Edelstein effect (IREE) in 1\u20133 monolayers (ML) to the inverse spin Hall effect (ISHE) in multilayers (&gt;3 ML) of PtSe\n                    <jats:sub>2<\/jats:sub>\n                    enabling the extraction of the perpendicular spin diffusion length and relative strength of IREE and ISHE is demonstrated. This band structure flexibility makes PtSe\n                    <jats:sub>2<\/jats:sub>\n                    an ideal candidate to explore the underlying mechanisms and engineering of the SCC as well as for the development of tuneable THz spintronic\u00a0emitters.\n                  <\/jats:p>","DOI":"10.1002\/adma.202304243","type":"journal-article","created":{"date-parts":[[2023,12,30]],"date-time":"2023-12-30T23:49:10Z","timestamp":1703980150000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":32,"title":["Atomic\u2010Layer Controlled Transition from Inverse Rashba\u2013Edelstein Effect to Inverse Spin Hall Effect in 2D PtSe\n                    <sub>2<\/sub>\n                    Probed by THz Spintronic Emission"],"prefix":"10.1002","volume":"36","author":[{"given":"Khasan","family":"Abdukayumov","sequence":"first","affiliation":[{"name":"CEA, CNRS, Universit\u00e9 Grenoble Alpes, Grenoble INP IRIG\u2010Spintec  Grenoble 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