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Here, reaction\u2010diffusion driven, immersion\u2010controlled patterning (R\u2010DIP) is introduced, a self\u2010organization strategy using immersion\u2010controlled reaction\u2010diffusion for targeted line patterning in thin films. By modulating immersion speeds, the movement of a reaction\u2010diffusion front over gel films is controlled, which induces precipitation of highly uniform lines at the reaction front. A balance between the immersion speed and diffusion provides both hands\u2010on tunability of the line spacing () as well as error\u2010correction against defects. This immersion\u2010driven patterning strategy is widely applicable, which is demonstrated by producing line patterns of silver\/silver oxide nanoparticles, silver chromate, silver dichromate, and lead carbonate. Through combinatorial stacking of different line patterns, hybrid materials with multi\u2010dimensional patterns such as square\u2010, diamond\u2010, rectangle\u2010, and triangle\u2010shaped motifs are fabricated. The functionality potential and scalability is demonstrated by producing both wafer\u2010scale diffraction gratings with user\u2010defined features as well as an opto\u2010mechanical sensor based on Moir\u00e9\u00a0patterning.<\/jats:p>","DOI":"10.1002\/adma.202305191","type":"journal-article","created":{"date-parts":[[2023,7,20]],"date-time":"2023-07-20T16:36:35Z","timestamp":1689870995000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":7,"title":["Patterning Complex Line Motifs in Thin Films Using Immersion\u2010Controlled Reaction\u2010Diffusion"],"prefix":"10.1002","volume":"35","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-4228-7316","authenticated-orcid":false,"given":"Christiaan T.","family":"van Campenhout","sequence":"first","affiliation":[{"name":"AMOLF Science Park 104 Amsterdam 1098XG The Netherlands"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hinco","family":"Schoenmaker","sequence":"additional","affiliation":[{"name":"AMOLF Science Park 104 Amsterdam 1098XG The Netherlands"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Martin","family":"van Hecke","sequence":"additional","affiliation":[{"name":"AMOLF Science Park 104 Amsterdam 1098XG The Netherlands"},{"name":"Leiden Institute of Physics Leiden University  Niels Bohrweg 2 CA Leiden 2333 The Netherlands"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0028-2354","authenticated-orcid":false,"given":"Willem L.","family":"Noorduin","sequence":"additional","affiliation":[{"name":"AMOLF Science Park 104 Amsterdam 1098XG The Netherlands"},{"name":"Van 't Hoff Institute for Molecular Sciences University of Amsterdam  Science Park 904 Amsterdam 1090 GD The Netherlands"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2023,8,2]]},"reference":[{"key":"e_1_2_8_1_1","volume-title":"The Self\u2010Made Tapestry: Pattern Formation in Nature","author":"Ball P.","year":"1999"},{"key":"e_1_2_8_2_1","doi-asserted-by":"publisher","DOI":"10.1038\/ncomms1970"},{"key":"e_1_2_8_3_1","doi-asserted-by":"publisher","DOI":"10.1088\/2040-8986\/aaff39"},{"key":"e_1_2_8_4_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.aat8297"},{"key":"e_1_2_8_5_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.201706654"},{"key":"e_1_2_8_6_1","doi-asserted-by":"publisher","DOI":"10.1039\/C5CS00533G"},{"key":"e_1_2_8_7_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41563-022-01384-1"},{"key":"e_1_2_8_8_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.201905554"},{"key":"e_1_2_8_9_1","doi-asserted-by":"publisher","DOI":"10.1039\/D2CP02542F"},{"key":"e_1_2_8_10_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.aav4299"},{"key":"e_1_2_8_11_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202001474"},{"key":"e_1_2_8_12_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41563-022-01223-3"},{"key":"e_1_2_8_13_1","volume-title":"Nanofabrication: Nanolithography Techniques and their Applications","author":"De Teresa J. 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