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Here, a functional unit combination strategy is proposed to design novel RTP molecules combining a folding unit with diverse luminescent cores. The different luminescent cores are mainly responsible for tunable RTP properties, while the folding unit contributes to the spin\u2013orbit coupling (SOC) enhancement, which makes the RTP material design as workable as the building block principle. By this strategy, a series of color\/lifetime\u2010tunable RTP materials is achieved with unique photo\u2010responsive RTP enhancement when subjected to UV irradiation, which expands their application scenarios in reusable privacy tags, advanced \u201c4D\u201d encryption, and phase separation analysis of blended polymers. This work suggests a simple and effective strategy to design purely organic RTP materials with tunable color and lifetime, and also provides new application options for photo\u2010responsive dynamic RTP materials.<\/jats:p>","DOI":"10.1002\/adma.202306784","type":"journal-article","created":{"date-parts":[[2023,10,2]],"date-time":"2023-10-02T07:00:31Z","timestamp":1696230031000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":87,"title":["Photo\u2010Responsive Dynamic Organic Room\u2010Temperature Phosphorescence Materials Based on a Functional Unit Combination Strategy"],"prefix":"10.1002","volume":"36","author":[{"given":"Zhiqiang","family":"Yang","sequence":"first","affiliation":[{"name":"State Key Laboratory of Supramolecular Structure and Materials College of Chemistry Jilin University  Changchun Jilin 130012 P. R. 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