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Electrocatalytic hydrogenation (ECH) using water as the hydrogen source has emerged as an alternative to conventional thermocatalytic processes for sustainable and decentralized chemical synthesis under mild conditions. Among the various ECH catalysts, copper\u2010based (Cu\u2010based) nanomaterials are promising candidates due to their earth\u2010abundance, unique electronic structure, versatility, and high activity\/selectivity. Herein, recent advances in the application of Cu\u2010based catalysts in ECH reactions for the upgrading of valuable chemicals are systematically analyzed. The unique properties of Cu\u2010based catalysts in ECH are initially introduced, followed by design strategies to enhance their activity and selectivity. Then, typical ECH reactions on Cu\u2010based catalysts are presented in detail, including carbon dioxide reduction for multicarbon generation, alkyne\u2010to\u2010alkene conversion, selective aldehyde conversion, ammonia production from nitrogen\u2010containing substances, and amine production from organic nitrogen compounds. In these catalysts, the role of catalyst composition and nanostructures toward different products is focused. The co\u2010hydrogenation of two substrates (e.g., CO\n                    <jats:sub>2<\/jats:sub>\n                    and NO\n                    <jats:italic>\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    <jats:sup>n<\/jats:sup>\n                    , SO\n                    <jats:sub>3<\/jats:sub>\n                    <jats:sup>2\u2013<\/jats:sup>\n                    , etc.) via C\u2500N, C\u2500S, and C\u2500C cross\u2010coupling reactions are also highlighted. Finally, the critical issues and future perspectives of Cu\u2010catalyzed ECH are proposed to accelerate the rational development of next\u2010generation catalysts.\n                  <\/jats:p>","DOI":"10.1002\/adma.202307913","type":"journal-article","created":{"date-parts":[[2023,9,27]],"date-time":"2023-09-27T14:15:51Z","timestamp":1695824151000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":118,"title":["Recent Advances in Electrocatalytic Hydrogenation Reactions on Copper\u2010Based Catalysts"],"prefix":"10.1002","volume":"36","author":[{"given":"Min","family":"Zheng","sequence":"first","affiliation":[{"name":"School of Chemical Engineering The University of Adelaide  Adelaide SA 5005 Australia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Junyu","family":"Zhang","sequence":"additional","affiliation":[{"name":"School of Chemical Engineering The University of Adelaide  Adelaide SA 5005 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