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However, it is challenging to realize the preparation of high\u2010toughness (with both high stress and strain) ionic elastomers. Herein, high\u2010toughness linear poly(ionic liquid) (PIL) elastomers are constructed via supramolecular ionic networks formed by the polymerization of halometallate ionic liquid (IL) monomers, without any chemical crosslinking. The obtained linear PIL elastomers exhibit high strength (16.5 MPa), Young's modulus (157.49 MPa), toughness (130.31 MJ m<jats:sup>\u22123<\/jats:sup>), and high crack propagation insensitivity (fracture energy 243.37 kJ m<jats:sup>\u22122<\/jats:sup>), owing to the enhanced intermolecular noncovalent interactions of PIL chains. Furthermore, PIL elastomer\u2010based strain, pressure, and touch sensors have shown high sensitivity. The linear noncovalent crosslinked network endows the PIL elastomers with self\u2010healing and recyclable properties, and broad application prospects in the fields of flexible sensor devices, health monitoring, and human\u2013machine interaction.<\/jats:p>","DOI":"10.1002\/adma.202308547","type":"journal-article","created":{"date-parts":[[2023,10,10]],"date-time":"2023-10-10T20:34:09Z","timestamp":1696970049000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":118,"title":["High\u2010Toughness and High\u2010Strength Solvent\u2010Free Linear Poly(ionic liquid) Elastomers"],"prefix":"10.1002","volume":"36","author":[{"given":"Lingling","family":"Li","sequence":"first","affiliation":[{"name":"Jiangsu Engineering Laboratory of Novel Functional Polymeric Materials Jiangsu Key Laboratory of Advanced Negative Carbon Technologies Suzhou Key Laboratory of Soft Material and New Energy College of Chemistry Chemical Engineering and 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