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For the Au\u2010coated Zn metal symmetric cell, uniform deposition of Zn\u2010derived compounds\u00a0was revealed by operando synchrotron tomography. Microscopic studies demonstrate that the Au\u2010coating layer is induced to form a new Zn\u2013Au alloy during the initial Zn deposition, resulting in stabilized long\u2010term stripping\/plating of Zn via the \u2018embracing effect\u2019 that intimately accommodates Zn deposition for further cycles. This property supports the successful operation of symmetrical cells up to 50 mA cm<jats:sup>\u22122<\/jats:sup>. According to Zn electrodeposition simulation, it is verified that the suppression of dendrite growth is responsible for the electro\u2010conducting Au nanolayer that uniformly distributes the electric field and protects the Zn electrode from corrosion, ultimately promoting uniform Zn growth. The compatibility of the Au\u2010coating layer for full cell configuration is verified using NaV<jats:sub>3<\/jats:sub>O<jats:sub>8<\/jats:sub> as a cathode material over 1\u00a0000 cycles. This finding provides a new pathway for the enhancement of the electrochemical performance of ZIBs by suppressing the dendritic growth of Zn by means of a zincophilic Au nanolayer.<\/jats:p>","DOI":"10.1002\/adma.202308592","type":"journal-article","created":{"date-parts":[[2023,11,11]],"date-time":"2023-11-11T20:39:26Z","timestamp":1699735166000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":39,"title":["Gold\u2010Nanolayer\u2010Derived Zincophilicity Suppressing Metallic Zinc Dendrites and Its Efficacy in Improving Electrochemical Stability of Aqueous Zinc\u2010Ion Batteries"],"prefix":"10.1002","volume":"36","author":[{"given":"Hee Jae","family":"Kim","sequence":"first","affiliation":[{"name":"Hybrid Materials Research Center Department of Nanotechnology and Advanced Materials Engineering &amp; Sejong Battery Institute Sejong University  Seoul 05006 South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Sun","family":"Kim","sequence":"additional","affiliation":[{"name":"Hybrid Materials Research Center Department of Nanotechnology and Advanced Materials Engineering &amp; Sejong Battery Institute Sejong University  Seoul 05006 South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Suhwan","family":"Kim","sequence":"additional","affiliation":[{"name":"Department of Energy Science and Engineering Daegu Gyeongbuk Institute of Science and Technology (DGIST)  Daegu 42988 South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Sungkyu","family":"Kim","sequence":"additional","affiliation":[{"name":"Hybrid Materials Research Center Department of Nanotechnology and Advanced Materials Engineering &amp; Sejong Battery Institute Sejong University  Seoul 05006 South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kwang","family":"Heo","sequence":"additional","affiliation":[{"name":"Hybrid Materials Research Center Department of Nanotechnology and Advanced Materials Engineering &amp; Sejong Battery Institute Sejong University  Seoul 05006 South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jae\u2010Hong","family":"Lim","sequence":"additional","affiliation":[{"name":"Pohang Accelerator Laboratory  80 Jigokro\u2010127\u2010beongil, Nam\u2010gu Pohang Gyeongbuk 37673 South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hitoshi","family":"Yashiro","sequence":"additional","affiliation":[{"name":"Department of Chemistry and Bioengineering Iwate University  4\u20103\u20105 Ueda Morioka Iwate 020\u20138551 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hyeon\u2010Ji","family":"Shin","sequence":"additional","affiliation":[{"name":"Center for Energy Storage Research Korea Institute of Science and Technology  Seoul 02792 South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hun\u2010Gi","family":"Jung","sequence":"additional","affiliation":[{"name":"Center for Energy Storage Research Korea Institute of Science and Technology  Seoul 02792 South Korea"},{"name":"KIST\u2010SKKU Carbon\u2010Neutral Research Center Sungkyunkwan University  Suwon 16419 South Korea"},{"name":"Department of Energy Science Sungkyunkwan University  Suwon 16419 South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2002-2218","authenticated-orcid":false,"given":"Yong Min","family":"Lee","sequence":"additional","affiliation":[{"name":"Department of Energy Science and Engineering Daegu Gyeongbuk Institute of Science and Technology (DGIST)  Daegu 42988 South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6888-5376","authenticated-orcid":false,"given":"Seung\u2010Taek","family":"Myung","sequence":"additional","affiliation":[{"name":"Hybrid Materials Research Center Department of Nanotechnology and Advanced Materials Engineering &amp; 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