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Persulfate\u2010based advanced oxidation processes (PS\u2010AOPs) have attracted much attention as they address potential water purification challenges. However, overcoming the mass transfer constraint and the catalyst's inherent site agglomeration in the heterogeneous system remains urgent. Herein, the abundant metal\u2010anchored loading (\u22486\u20138\u00a0g m\n                    <jats:sup>\u22122<\/jats:sup>\n                    ) of alginate hydrogel membranes coupled with cross\u2010flow mode as an efficient strategy for water purification applications is proposed. The organic flux of the confined hydrogel interfaces sharply enlarges with the reduction of the thickness of the boundary layer via the pressure field. The normalized property of the system displays a remarkable organic (sulfonamides) elimination rate of 4.87 \u00d7 10\n                    <jats:sup>4<\/jats:sup>\n                    \u00a0mg min\n                    <jats:sup>\u22121<\/jats:sup>\n                    mol\n                    <jats:sup>\u22121<\/jats:sup>\n                    . Furthermore, due to the fast reaction time (&lt;1\u00a0min), cross\u2010flow mode only reaches a meager energy cost (\u22482.21\u00a0Wh m\n                    <jats:sup>\u22123<\/jats:sup>\n                    ) under the pressure drive field. It is anticipated that this finding provides insight into the novel design with ultrafast organic removal performance and low techno\u2010economic cost (i.e., energy operation cost, material, and reagent cost) for the field of water purification under various PS\u2010AOPs challenging scenarios.\n                  <\/jats:p>","DOI":"10.1002\/adma.202311416","type":"journal-article","created":{"date-parts":[[2024,1,22]],"date-time":"2024-01-22T20:36:05Z","timestamp":1705955765000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":34,"title":["Sustainable and Rapid Water Purification at the Confined Hydrogel Interface"],"prefix":"10.1002","volume":"36","author":[{"given":"Min","family":"Chen","sequence":"first","affiliation":[{"name":"State Key Laboratory of Separation Membranes and Membrane Processes\/National Centre for International Joint Research on Separation Membranes Tiangong University  Tianjin 300387 P. R. 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