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The severe Coffee\u2010ring effect (CRE) is considered to be the primary reason for the nonuniform distribution of active layer films. To solve this key printing problem, the cosolvent strategy is presented to deposit the active layer films. The guest solvent Mesitylene with a higher boiling point and a lower surface tension is incorporated into the host solvent o\u2010XY to optimize the rheological properties, such as surface tension and viscosity of the active layer solutions. And the synergistic effect of inward Marangoni flow generation and solution thickening caused by the cosolvent strategy can effectively restrain CRE, resulting in highly homogeneous large\u2010area active layer films. In addition, the optimized crystallization and phase separation of active layer films effectively accelerate the charge transport and exciton dissociation of devices. Consequently, based on PM6:BTP\u2010eC9 system, the device prepared with the co\u2010solvent strategy shows the a power conversion efficiency of 17.80%. Moreover, as the effective area scales to 1 and 16.94 cm<jats:sup>2<\/jats:sup>, the recorded performances are altered to 16.71% and 14.58%. This study provides a universal pathway for the development of green\u2010printed high\u2010efficiency organic photovoltaics.<\/jats:p>","DOI":"10.1002\/adma.202313098","type":"journal-article","created":{"date-parts":[[2024,2,10]],"date-time":"2024-02-10T11:29:27Z","timestamp":1707564567000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":55,"title":["Green Printing for Scalable Organic Photovoltaic Modules by Controlling the Gradient Marangoni Flow"],"prefix":"10.1002","volume":"36","author":[{"given":"Hanlin","family":"Wang","sequence":"first","affiliation":[{"name":"School of Physics and Materials Science\/Institute of Polymers and Energy Chemistry (IPEC)\/Film Energy Chemistry for Jiangxi Provincial Key Laboratory (FEC) Nanchang University 999 Xuefu Avenue Nanchang 330031 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Siqi","family":"Liu","sequence":"additional","affiliation":[{"name":"College of 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