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Despite considerable efforts, developing scalable, high\u2010performance underwater adhesives through a simple and effective method remains a formidable challenge. This study presents a novel mesh\u2010tailoring strategy for in situ, rapid, and ultrastrong oleogel\u2010based underwater adhesives (OUA), which comprises a highly crosslinked polyurethane network with a matching mesh size (\u22482.22\u00a0nm) that precisely entraps bio\u2010based epoxidized soybean oil (ESO) molecules (\u22482.31\u00a0nm) by steric hindrance effect. This oleogel exhibits unprecedented robust mechanical properties (\u224835\u00a0MPa) and maintains stability under extreme conditions, including high temperatures (100\u00a0\u00b0C), high pressures (30\u00a0MPa), and immersion in various solvents (water, ethanol, or ESO). In particular, this oleogel displays high hydrophobicity, rapid curing, and strong interface affinity, resulting in ultrahigh underwater adhesion strength (up to 2.13\u00a0MPa) and exceptional substrate universality. Moreover, the remarkable environmental adaptability and stability of OUA enable its use in harsh aqueous environments, including acidic\/alkaline, saline, and extreme temperature solutions. The comprehensive capabilities of the OUA underscore its potential for building underwater structures, repairing leaky containers, and sealing broken submarine pipelines. This research establishes the foundation for the designing of next\u2010generation underwater adhesives and offers fresh perspectives for exploring oleogel\u2010based materials.<\/jats:p>","DOI":"10.1002\/adma.202313495","type":"journal-article","created":{"date-parts":[[2024,4,29]],"date-time":"2024-04-29T14:56:10Z","timestamp":1714402570000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":57,"title":["Sterically Hindered Oleogel\u2010Based Underwater Adhesive Enabled by Mesh\u2010Tailoring Strategy"],"prefix":"10.1002","volume":"36","author":[{"given":"Bin","family":"Zhang","sequence":"first","affiliation":[{"name":"Faculty of Materials Science and Engineering South China University of Technology  Guangzhou 510640 P. R. 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