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In this regard, short peptide\u2010based self\u2010assembled hydrogels show promising potential to act as bioinspired supramolecular substrates for developing tactile sensors showing biocompatibility and biodegradability. However, the intrinsic difficulty to modulate the mechanical properties severely restricts their extensive employment. Herein, by controlling the self\u2010assembly of 9\u2010fluorenylmethoxycarbonyl\u2010modifid diphenylalanine (Fmoc\u2010FF) through introduction of polyethylene glycol diacrylate (PEGDA), wider nanoribbons are achieved by untwisting from well\u2010established thinner nanofibers, and the mechanical properties of the supramolecular hydrogels can be enhanced 10\u2010fold, supplying bioinspired supramolecular encapsulating substrate for tactile sensing. Furthermore, by doping with poly(3,4\u2010ethylenedioxythiophene):poly(styrene sulfonate) (PEDOT:PSS) and 9\u2010fluorenylmethoxycarbonyl\u2010modifid 3,4\u2010dihydroxy\u2010<jats:sc>l<\/jats:sc>\u2010phenylalanine (Fmoc\u2010DOPA), the Fmoc\u2010FF self\u2010assembled hydrogels can be engineered to be conductive and adhesive, providing bioinspired sensing units and adhesive layer for tactile sensing applications. Therefore, the integration of these modules results in peptide hydrogelation\u2010based tactile sensors, showing high sensitivity and sustainable responses with intrinsic biocompatibility and biodegradability. The findings establish the feasibility of developing programmable peptide self\u2010assembly with adjustable features for tactile sensing applications.<\/jats:p>","DOI":"10.1002\/adma.202401678","type":"journal-article","created":{"date-parts":[[2024,4,28]],"date-time":"2024-04-28T04:09:41Z","timestamp":1714277381000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":37,"title":["Bioinspired Flexible Hydrogelation with Programmable Properties for Tactile Sensing"],"prefix":"10.1002","volume":"36","author":[{"given":"Yunxiao","family":"Wang","sequence":"first","affiliation":[{"name":"State Key Laboratory of Fluid Power and Mechatronic Systems Key Laboratory of Advanced Manufacturing Technology of Zhejiang Province School of Mechanical Engineering Zhejiang University  Hangzhou 310058 China"},{"name":"Zhejiang\u2010Israel Joint Laboratory of Self\u2010Assembling Functional Materials ZJU\u2010Hangzhou Global Scientific and 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