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However, solution\u2010printed OSCFs are typically plagued by the existence of abundant structural defects, which pose a formidable challenge to achieving large\u2010scale and high\u2010performance organic electronics. Here, it is elucidated that these structural defects are mainly originated from printing flow\u2010induced anisotropic growth, an important factor that is overlooked for too long. In light of this, a surfactant\u2010additive printing method is proposed to effectively overcome the anisotropic growth, enabling the deposition of uniform OSCFs over the wafer scale at a high speed of 1.2 mm s<jats:sup>\u22121<\/jats:sup> at room temperature. The resulting OSCF exhibits appealing performance with a high average mobility up to 10.7 cm<jats:sup>2<\/jats:sup> V<jats:sup>\u22121<\/jats:sup> s<jats:sup>\u22121<\/jats:sup>, which is one of the highest values for flexible organic field\u2010effect transistor arrays. Moreover, large\u2010scale OSCF\u2010based flexible logic circuits, which can be bent without degradation to a radius as small as 4.0 mm and over 1000 cycles are realized. The work provides profound insights into breaking the limitation of flow\u2010induced anisotropic growth and opens new avenues for printing large\u2010scale organic single\u2010crystal electronics.<\/jats:p>","DOI":"10.1002\/adma.202401822","type":"journal-article","created":{"date-parts":[[2024,3,31]],"date-time":"2024-03-31T11:00:15Z","timestamp":1711882815000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":34,"title":["Breaking Fundamental Limitation of Flow\u2010Induced Anisotropic Growth for Large\u2010Scale and Fast Printing of Organic Single\u2010Crystal Films"],"prefix":"10.1002","volume":"36","author":[{"given":"Fangming","family":"Sheng","sequence":"first","affiliation":[{"name":"Institute of Functional Nano &amp; Soft Materials (FUNSOM) Jiangsu Key Laboratory for Carbon\u2010Based Functional Materials &amp; Devices Soochow University  Suzhou Jiangsu 215123 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0067-0624","authenticated-orcid":false,"given":"Wei","family":"Deng","sequence":"additional","affiliation":[{"name":"Institute of Functional Nano &amp; 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