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The limitation remains; however, that an additional tunneling contact resistance occurs owing to the inherent vdW gap between the metal and the semiconductor. Here, it is demonstrated from theoretical calculations that stronger non\u2010covalent hydrogen\u2010bonding interactions facilitate electron tunneling and significantly reduce the contact resistance; thus, promising to break the limitations of the vdW contact. \u03c0\u2010plane hydrogen\u2010bonding contacts in surface\u2010engineered MXene\/carbon nanotube metal\/semiconductor heterojunctions are realized, and an anomalous temperature\u2010dependent tunneling resistance is observed. Low\u2010dimensional flexible thin\u2010film transistors integrated by hydrogen\u2010bonding contacts exhibit both excellent flexibility and carrier mobility orders of magnitude higher than their counterparts with vdW contacts. This strategy demonstrates a scalable solution for realizing high\u2010performance and low\u2010power flexible electronics beyond vdW contacts.<\/jats:p>","DOI":"10.1002\/adma.202404626","type":"journal-article","created":{"date-parts":[[2024,6,3]],"date-time":"2024-06-03T00:53:30Z","timestamp":1717376010000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":18,"title":["Hydrogen\u2010Bonding Integrated Low\u2010Dimensional Flexible Electronics Beyond the Limitations of van der Waals Contacts"],"prefix":"10.1002","volume":"36","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-5387-4981","authenticated-orcid":false,"given":"Dexing","family":"Liu","sequence":"first","affiliation":[{"name":"School of Electronic and Computer Engineering Peking University  Shenzhen 518055 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ziyi","family":"Liu","sequence":"additional","affiliation":[{"name":"School of Electronic and Computer Engineering Peking University  Shenzhen 518055 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xinyu","family":"Gao","sequence":"additional","affiliation":[{"name":"School of Electronic and Computer Engineering Peking University  Shenzhen 518055 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jiahao","family":"Zhu","sequence":"additional","affiliation":[{"name":"School of Electronic and Computer Engineering Peking University  Shenzhen 518055 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zifan","family":"Wang","sequence":"additional","affiliation":[{"name":"School of Electronic and Computer Engineering Peking University  Shenzhen 518055 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Rui","family":"Qiu","sequence":"additional","affiliation":[{"name":"School of Electronic and Computer Engineering Peking University  Shenzhen 518055 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qinqi","family":"Ren","sequence":"additional","affiliation":[{"name":"School of Electronic and Computer Engineering Peking University  Shenzhen 518055 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yiming","family":"Zhang","sequence":"additional","affiliation":[{"name":"School of Electronic and Computer Engineering Peking University  Shenzhen 518055 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shengdong","family":"Zhang","sequence":"additional","affiliation":[{"name":"School of Electronic and Computer Engineering Peking University  Shenzhen 518055 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2225-8024","authenticated-orcid":false,"given":"Min","family":"Zhang","sequence":"additional","affiliation":[{"name":"School of Electronic and Computer Engineering Peking University  Shenzhen 518055 China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2024,6,21]]},"reference":[{"key":"e_1_2_9_1_1","first-page":"367","volume":"113","author":"Schottky W.","year":"1939","journal-title":"Z. 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