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Strategies to reconcile environment\u2010triggered actuation and self\u2010powered sensing responses to different stimuli remain challenging. By tuning the in situ vapor phase solvent exchange effect in continuous electrospinning, an asymmetric highly\u2010aligned all\u2010fiber membrane (HAFM) with a hierarchical \u201cgrape\u2010like\u201d nanosphere\u2010assembled microfiber structure (specific surface area of 13.6\u00a0m\n                    <jats:sup>2\u00a0<\/jats:sup>\n                    g\n                    <jats:sup>\u22121<\/jats:sup>\n                    ) and excellent mechanical toughness (tensile stress of 5.5\u00a0MPa, and fracture toughness of 798\u00a0KJ\u00a0m\n                    <jats:sup>\u22123<\/jats:sup>\n                    ) is developed, which shows efficient asymmetric actuation to both photothermal and humidity stimuli. The HAFM consists of a metal\u2010organic framework (MOF)\u2010enhanced moisture\u2010responsive layer and an MXene\u2010improved photothermal\u2010responsive layer, which achieves substantial actuation with a bending curvature up to \u22487.23\u00a0cm\n                    <jats:sup>\u22121<\/jats:sup>\n                    and a fast response of 0.60\u00a0cm\n                    <jats:sup>\u22121<\/jats:sup>\n                    \u00a0s\n                    <jats:sup>\u22121<\/jats:sup>\n                    . By tailoring the fiber alignment and bi\u2010layer thickness ratio, different types of micromanipulators, automatic walking robots, and plant robots with programmable structures are demonstrated, which are realized for self\u2010powered information perception of material type, object moisture, and temperature by integrating the autonomous triboelectric effect induced by photothermal\u2010moisture actuation. This work presents fiber materials with programable hierarchical asymmetries and inspires a common strategy for self\u2010powered organism\u2010interface robots to interact with complex environments.\n                  <\/jats:p>","DOI":"10.1002\/adma.202404696","type":"journal-article","created":{"date-parts":[[2024,6,26]],"date-time":"2024-06-26T06:29:43Z","timestamp":1719383383000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":53,"title":["Highly\u2010Aligned All\u2010Fiber Actuator with Asymmetric Photothermal\u2010Humidity Response and Autonomous Perceptivity"],"prefix":"10.1002","volume":"36","author":[{"given":"Yufan","family":"Zhang","sequence":"first","affiliation":[{"name":"State Key Laboratory for Modification of Chemical Fibers and Polymer Materials Innovation Center for Textile Science and Technology and College of Textiles Donghua University  Shanghai 201620 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201620 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yue","family":"Zhang","sequence":"additional","affiliation":[{"name":"State Key Laboratory for Modification of Chemical Fibers and Polymer Materials Innovation Center for Textile Science and Technology and College of Textiles Donghua University  Shanghai 201620 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Mengjie","family":"Wu","sequence":"additional","affiliation":[{"name":"State Key Laboratory for Modification of Chemical Fibers and Polymer Materials Innovation Center for Textile Science and Technology and College of Textiles Donghua University  Shanghai 201620 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zeren","family":"Lu","sequence":"additional","affiliation":[{"name":"College of Materials Science and Engineering Donghua University  Shanghai 201620 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