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Here, heavy\u2010atom effect is introduced first to construct ICz\u2010MR emitter using a sulfur\u2010containing substitute, simultaneously enhancing both spin\u2013orbit and spin\u2013vibronic coupling to afford a fast RISC with a rate of 1.2\u00a0\u00d7\u00a010\n                    <jats:sup>5<\/jats:sup>\n                    \u00a0s\n                    <jats:sup>\u22121<\/jats:sup>\n                    , nearly one order of magnitude higher than previous maximum values. The emitter also exhibits an extremely narrow deep\u2010blue emission peaking at 456\u00a0nm with full\u2010width at half\u2010maxima of merely 12\u00a0nm and a photoluminescence quantum yield of 92%. Benefiting from its efficient triplet upconversion capability, this emitter achieves not only a high maximum external quantum efficiency (EQE) of 31.1% in organic light\u2010emitting diodes but also greatly alleviates efficiency roll\u2010off, affording record\u2010high EQEs of 29.9% at 1000\u00a0cd\u00a0m\n                    <jats:sup>\u22122<\/jats:sup>\n                    and 18.7% at 5000\u00a0cd\u00a0m\n                    <jats:sup>\u22122<\/jats:sup>\n                    among devices with ICz\u2010MR emitters.\n                  <\/jats:p>","DOI":"10.1002\/adma.202408816","type":"journal-article","created":{"date-parts":[[2024,9,17]],"date-time":"2024-09-17T12:10:51Z","timestamp":1726575051000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":56,"title":["Enhancing Spin\u2013Orbit Coupling in an Indolocarbazole Multiresonance Emitter by a Sulfur\u2010Containing Peripheral Substituent for a Fast Reverse Intersystem Crossing"],"prefix":"10.1002","volume":"36","author":[{"given":"Tianjiao","family":"Fan","sequence":"first","affiliation":[{"name":"Key Lab of Organic Optoelectronics and Molecular Engineering of Ministry of Education Department of Chemistry Tsinghua University  Beijing 100084 P. 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