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Light\u2010based tomographic manufacturing enables spatial\u2010selective polymerization of a bioresin, resulting in higher throughput and resolution than what is achieved using traditional techniques. However, methods for multi\u2010material printing are needed for broad VBP adoption and applicability. Although converging VBP with extrusion bioprinting in support baths offers a novel, promising solution, further knowledge on the engineering of hydrogels as light\u2010responsive, volumetrically printable baths is needed. Therefore, this study investigates the tuning of gelatin macromers, in particular leveraging the effect of molecular weight and degree of modification, to overcome these challenges, creating a library of materials for VBP and Embedded extrusion Volumetric Printing (EmVP). Bioresins with tunable printability and mechanical properties are produced, and a novel subset of gelatins and GelMA exhibiting stable shear\u2010yielding behavior offers a new, single\u2010component, ready\u2010to\u2010use suspension medium for in\u2010bath printing, which is stable over multiple hours without needing temperature control. As a proof\u2010of\u2010concept biological application, bioprinted gels are tested with insulin\u2010producing pancreatic cell lines for 21 days of culture. Leveraging a multi\u2010color printer, complex multi\u2010material and multi\u2010cellular geometries are produced, enhancing the accessibility of volumetric printing for advanced tissue models.<\/jats:p>","DOI":"10.1002\/adma.202409355","type":"journal-article","created":{"date-parts":[[2025,3,12]],"date-time":"2025-03-12T02:38:12Z","timestamp":1741747092000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":39,"title":["Multi\u2010material Volumetric Bioprinting and Plug\u2010and\u2010play Suspension Bath Biofabrication via Bioresin Molecular Weight Tuning and via Multiwavelength Alignment Optics"],"prefix":"10.1002","volume":"37","author":[{"given":"Davide","family":"Ribezzi","sequence":"first","affiliation":[{"name":"Department of Orthopaedics University Medical Center Utrecht Utrecht University  Utrecht 3584 CX The 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