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Magnetotransport is generally sensitive to magnetic field orientations. In contrast, efficient and isotropic modulation of electronic transport, which is useful in technology applications such as omnidirectional sensing, is rarely seen, especially for pristine crystals. Here a strategy is proposed to realize extremely strong modulation of electron conduction by magnetic field which is independent of field direction. GdPS, a layered antiferromagnetic semiconductor with resistivity anisotropies, supports a field\u2010driven insulator\u2010to\u2010metal transition with a paradoxically isotropic gigantic negative magnetoresistance insensitive to magnetic field orientations. This isotropic magnetoresistance originates from the combined effects of a near\u2010zero spin\u2013orbit coupling of Gd\n                    <jats:sup>3+<\/jats:sup>\n                    \u2010based half\u2010filling\n                    <jats:italic>f<\/jats:italic>\n                    \u2010electron system and the strong on\u2010site\n                    <jats:italic>f<\/jats:italic>\n                    \u2013\n                    <jats:italic>d<\/jats:italic>\n                    exchange coupling in Gd atoms. These results not only provide\u00a0a novel material system with extraordinary magnetotransport that offers a missing block for antiferromagnet\u2010based ultrafast and efficient spintronic devices, but also demonstrate the key ingredients for designing magnetic materials with desired transport properties for advanced functionalities.\n                  <\/jats:p>","DOI":"10.1002\/adma.202410655","type":"journal-article","created":{"date-parts":[[2024,10,12]],"date-time":"2024-10-12T01:43:41Z","timestamp":1728697421000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":10,"title":["Insulator\u2010to\u2010Metal Transition and Isotropic Gigantic Magnetoresistance in Layered Magnetic Semiconductors"],"prefix":"10.1002","volume":"36","author":[{"ORCID":"https:\/\/orcid.org\/0009-0006-8373-4529","authenticated-orcid":false,"given":"Gokul","family":"Acharya","sequence":"first","affiliation":[{"name":"Department of Physics University of Arkansas  Fayetteville AR 72701 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Bimal","family":"Neupane","sequence":"additional","affiliation":[{"name":"Department of Physics University of North Texas  Denton TX 76205 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chia\u2010Hsiu","family":"Hsu","sequence":"additional","affiliation":[{"name":"Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University  Singapore 637371 Singapore"},{"name":"Quantum Materials Science Unit Okinawa Institute of Science and Technology (OIST)  Okinawa 904\u20100495 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xian P.","family":"Yang","sequence":"additional","affiliation":[{"name":"Laboratory for Topological Quantum Matter and Advanced Spectroscopy (B7) Department of Physics Princeton University  Princeton NJ 08544 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"David","family":"Graf","sequence":"additional","affiliation":[{"name":"National High Magnetic Field Lab  Tallahassee FL 32310 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Eun Sang","family":"Choi","sequence":"additional","affiliation":[{"name":"National High Magnetic Field Lab  Tallahassee FL 32310 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Krishna","family":"Pandey","sequence":"additional","affiliation":[{"name":"Materials Science and Engineering Program Institute for Nanoscience and Engineering University of Arkansas  Fayetteville AR 72701 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Md Rafique Un","family":"Nabi","sequence":"additional","affiliation":[{"name":"Department of Physics University of Arkansas  Fayetteville AR 72701 USA"},{"name":"MonArk NSF Quantum Foundry University of Arkansas  Fayetteville AR 72701 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Santosh Karki","family":"Chhetri","sequence":"additional","affiliation":[{"name":"Department of Physics University of Arkansas  Fayetteville AR 72701 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Rabindra","family":"Basnet","sequence":"additional","affiliation":[{"name":"Department of Physics University of Arkansas  Fayetteville AR 72701 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Sumaya","family":"Rahman","sequence":"additional","affiliation":[{"name":"Materials Science and Engineering Program Institute for Nanoscience and Engineering University of Arkansas  Fayetteville AR 72701 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jian","family":"Wang","sequence":"additional","affiliation":[{"name":"Department of Chemistry and Biochemistry Wichita State University  Wichita KS 67260 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhengxin","family":"Hu","sequence":"additional","affiliation":[{"name":"Center for Basic Research on Materials National Institute for Materials Science (NIMS)  Tsukuba\u2010city Ibaraki 305\u20100047 Japan"},{"name":"Department of Chemistry University of Cambridge  Cambridge CB2 1EW UK"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Bo","family":"Da","sequence":"additional","affiliation":[{"name":"Center for Basic Research on Materials National Institute for Materials Science (NIMS)  Tsukuba\u2010city Ibaraki 305\u20100047 Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hugh O. 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