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However, though the INCI formation is regularly considered to improve the device performance by literature, there is no feasible approach to directly and reliably characterizing its formation in practical\u2010OSC films thus far. Here in this study, by theoretical analysis and calculation, the generation of INCIs in OSCs is found, normally consisting of relatively heavy elements, such as O\u00b7\u00b7\u00b7Se, O\u00b7\u00b7\u00b7S, N\u00b7\u00b7\u00b7S interactions, etc., can induce enhanced strength of spin\u2010orbit coupling, the primary factor dominating spin lifetime in OSCs. Based on this newly discovered theory, spin lifetime is creatively employed as a probe for sensitively detecting INCIs in OSC films via spin valves or field\u2010induced electron paramagnetic resonance, respectively. This study will highly promote academic and applicable developments of the cross\u2010cutting frontier research field between organic spintronics and electronics.\n                  <\/jats:p>","DOI":"10.1002\/adma.202410695","type":"journal-article","created":{"date-parts":[[2024,10,25]],"date-time":"2024-10-25T01:31:02Z","timestamp":1729819862000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":9,"title":["Spin\u2010Lifetime Probe for Detecting Intramolecular Noncovalent Interaction in Organic Semiconductors"],"prefix":"10.1002","volume":"36","author":[{"given":"Tingting","family":"Yang","sequence":"first","affiliation":[{"name":"Key Laboratory of Nanosystem and Hierarchical Fabrication CAS Center for Excellence in Nanoscience National Center for Nanoscience and Technology  Beijing 100190 P. R. 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