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The textbook routes employ quantum well states or Shockley\/topological type surface states whose spin degeneracy is lifted by strong spin\u2010orbit coupling and inversion symmetry breaking at the surface\/interface. The resultant spin polarization is usually truncated because of the intertwining between multiple orbitals. Here a unique type of surface states is realized, namely, dangling bond surface states in a family of ternary rare\u2010earth pnictide tellurides RePnTe (Re = La, Gd, Ce; Pn = Sb, Bi), with robust band structure and sizeable spin splitting. Spin and angle\u2010resolved photoemission spectroscopy measurements reveal high spin polarization and distinct spin\u2010momentum locking texture, which, according to the theoretical analysis, arise from local site asymmetry and surface\u2010purified spin\u2010orbital texture. The work extends the so\u2010called \u201chidden spin polarization\u201d from the bulk to the surface, presenting an intriguing spin\u2010orbital\u2010momentum\u2010layer locking phenomenon, which may shed lights on potential spintronic applications.<\/jats:p>","DOI":"10.1002\/adma.202411733","type":"journal-article","created":{"date-parts":[[2024,11,8]],"date-time":"2024-11-08T01:21:22Z","timestamp":1731028882000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":6,"title":["Observation of Highly Spin\u2010Polarized Dangling Bond Surface States in Rare\u2010Earth Pnictide Tellurides"],"prefix":"10.1002","volume":"37","author":[{"given":"Yongqing","family":"Cai","sequence":"first","affiliation":[{"name":"Songshan Lake Materials Laboratory  Dongguan 523808 China"},{"name":"School of Physics Dalian University of Technology  Dalian 116024 China"},{"name":"Department of Physics and Shenzhen Institute for Quantum Science and 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