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Solar energy, as an ideal sustainable resource, has significant potential to contribute to the goal of net\u2010zero carbon emissions if effectively harnessed and converted into a reliable and storable form of energy. Photocatalysts have the potential to convert sunlight into chemical energy carriers. In this respect, covalent organic frameworks (COFs) have shown great promise due to their tunable structure on different length scales, high surface areas, and beneficial optical properties such as broad visible light absorption. This review offers a comprehensive overview of the key developments in COF\u2010based photocatalysts for various applications, including water splitting, hydrogen peroxide generation, organic transformations, and carbon dioxide and nitrogen reduction. The underlying mechanisms, essential principles for material design, and structure\u2010function relationships of COFs in various photocatalytic applications are discussed. 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