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However, membrane fouling is a major challenge for conventional separation methods, leading to decreased efficiency and increased maintenance costs. Herein, a novel approach is reported by constructing liquid\u2010like surfaces with double anti\u2010fouling structure, incorporating soft nanomicelles within a rigid, chemically cross\u2010linked network for both anti\u2010membrane\u2010fouling and effective viscous water\u2010in\u2010oil emulsion separation. The coating significantly outperforms perfluorinated and commercial polytetrafluoroethylene (PVDF) membranes, effectively preventing the adhesion of viscous oils like crude oil and pump oil, and alleviating severe membrane fouling. For high\u2010viscosity emulsions (97.3 cP and 52.8 cP), it maintains over 99% separation efficiency after 3\u00a0h continuous use. Even after 15\u00a0h immersion in strong acids, alkalis, salts, or organic solvents, its separation efficiency remains above 95%. In addition, thanks to the anti\u2010membrane\u2010fouling ability, this work achieved 6\u00a0h continuous emulsion separation performance for the first time, demonstrating unparalleled long\u2010term stability. Overall, this study offers valuable insights into the development of innovative coatings for efficient and eco\u2010friendly separation of high\u2010viscosity emulsions.<\/jats:p>","DOI":"10.1002\/adma.202413751","type":"journal-article","created":{"date-parts":[[2024,12,9]],"date-time":"2024-12-09T01:50:57Z","timestamp":1733709057000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":50,"title":["Ultra\u2010Antifouling Liquid\u2010Like Surfaces for Sustainable Viscous Water\u2010in\u2010Oil Emulsions Separation and Oil Recovery"],"prefix":"10.1002","volume":"37","author":[{"given":"Weiwei","family":"Zheng","sequence":"first","affiliation":[{"name":"College of Chemical Engineering Fuzhou University  Fuzhou 350116 P. R. 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