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However, limited capacities, high charge overpotentials, and short lifetime are troubling obstacles for realizing their real\u2010world implementation. Common strategies, including introducing solid\u2010state catalysts (SSCs) and redox mediators (RMs), are insufficient to solve these issues. Herein, Ru\u2010loaded amino\u2010phenanthroline\u2010based carbonized polymer dots (RuApCPDs) integrating the catalytic activity of SSCs with the mobility of RMs have been designed to behave as quasi\u2010homogeneous catalysts in the electrolyte. Their mobile nature can ensure the avoidance of complete coverage of active sites, and the catalytic ability decreases the charge overpotential through co\u2010deposition with the discharge products. Additionally, the RuApCPDs can also adjust the Li\n                    <jats:sup>+<\/jats:sup>\n                    solvation structure and well protect the Li metal anodes with high stability. As a result, the introduction of RuApCPDs leads to a fivefold increase in discharge capacity, a low charge voltage of 3.75 V, and a running life of 168 cycles (79 cycles without RuApCPDs). The multifunctional quasi\u2010homogeneous catalyst developed here demonstrates its advantageous potential as a new catalytic strategy for bringing Li\u2010O\n                    <jats:sub>2<\/jats:sub>\n                    batteries to become a viable technology.\n                  <\/jats:p>","DOI":"10.1002\/adma.202413948","type":"journal-article","created":{"date-parts":[[2024,12,29]],"date-time":"2024-12-29T22:47:02Z","timestamp":1735512422000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":19,"title":["Multifunctional Quasi\u2010Homogeneous Catalysts as a New Catalytic Strategy to Boost the Performance of Li\u2010O\n                    <sub>2<\/sub>\n                    Batteries"],"prefix":"10.1002","volume":"37","author":[{"given":"Haoran","family":"Zhang","sequence":"first","affiliation":[{"name":"State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied Chemistry Chinese Academy of Sciences  Changchun 130022 China"},{"name":"School of Applied Chemistry and Engineering University of Science and Technology of China  Hefei 230026 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yue","family":"Yu","sequence":"additional","affiliation":[{"name":"Department of Chemistry and Waterloo Institute for Nanotechnology University of Waterloo 200 University Ave. W.  Waterloo Ontario N2L 3G1 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Dongyue","family":"Yang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied Chemistry Chinese Academy of Sciences  Changchun 130022 China"},{"name":"School of Applied Chemistry and Engineering University of Science and Technology of China  Hefei 230026 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yingqi","family":"Fan","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied Chemistry Chinese Academy of Sciences  Changchun 130022 China"},{"name":"School of Applied Chemistry and Engineering University of Science and Technology of China  Hefei 230026 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hao","family":"Chen","sequence":"additional","affiliation":[{"name":"State Key Laboratory 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