{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,14]],"date-time":"2026-10-14T15:51:07Z","timestamp":1791993067927,"version":"4.4.0"},"reference-count":62,"publisher":"Wiley","issue":"18","license":[{"start":{"date-parts":[[2025,3,23]],"date-time":"2025-03-23T00:00:00Z","timestamp":1742688000000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"}],"funder":[{"DOI":"10.13039\/501100012166","name":"National Key Research and Development Program of China","doi-asserted-by":"publisher","award":["2022YFA1402600"],"award-info":[{"award-number":["2022YFA1402600"]}],"id":[{"id":"10.13039\/501100012166","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100021171","name":"Basic and Applied Basic Research Foundation of Guangdong Province","doi-asserted-by":"publisher","award":["2022A1515140117"],"award-info":[{"award-number":["2022A1515140117"]}],"id":[{"id":"10.13039\/501100021171","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["advanced.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Advanced Materials"],"published-print":{"date-parts":[[2025,5]]},"abstract":"<jats:title>Abstract<\/jats:title><jats:p>Strongly correlated magnets, exhibiting distinctive spin properties such as spin\u2010orbit coupling, spin polarization, and chiral spin, are regarded as the next\u2010generation high\u2010density magnetic storage materials in spintronics. Nevertheless, owing to intricate spin interactions, realizing controllable spin arrangement and high\u2010density magnetic storage remains a formidable challenge. Here, controllable multiple spin states induced by the baromagnetic effect in kagome lattice magnet Mn\u2083GaC are first reported, achieved by manipulating spin rotation within the spin\u2010polarized plane employing pressure. Neutron diffraction refinement and specific heat measurements under pressure, combined with first\u2010principles calculations, demonstrate that multiple spin states are originating from the synergistic mechanism between spin frustration and spin polarization related to the lifting of degeneracy in electronic microstates. Electrical transport measurements under pressure reveal that multiple spin states exhibit giant baro\u2010magnetoresistance effect, enabling enhanced storage density in spintronics via multi\u2010logic state applications. Integrating the pressure response and microscopic behaviors of spins, a comprehensive <jats:italic>p<\/jats:italic>\u2010<jats:italic>T<\/jats:italic>\u2010<jats:italic>H<\/jats:italic> phase diagram is constructed, offering a novel and robust framework for multi\u2010logic states. These findings provide critical insights into controllable spin states, opening a new avenue for high\u2010density magnetic storage through multiple spin states.<\/jats:p>","DOI":"10.1002\/adma.202420502","type":"journal-article","created":{"date-parts":[[2025,3,24]],"date-time":"2025-03-24T05:52:11Z","timestamp":1742795531000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":5,"title":["Emergent Multiple Spin States From Baromagnetic Effect in Strongly Correlated Magnet Mn\u2083GaC"],"prefix":"10.1002","volume":"37","author":[{"given":"Shihai","family":"An","sequence":"first","affiliation":[{"name":"School of Physics Beihang University  Beijing 100191 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Fan","family":"Yang","sequence":"additional","affiliation":[{"name":"School of Physics Beihang University  Beijing 100191 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2165-1593","authenticated-orcid":false,"given":"Ying","family":"Sun","sequence":"additional","affiliation":[{"name":"School of Physics Beihang University  Beijing 100191 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Sihao","family":"Deng","sequence":"additional","affiliation":[{"name":"Institute of High Energy Physics Chinese Academy of Sciences  Beijing 100049 China"},{"name":"Spallation Neutron Source Science Center  Dongguan 523803 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiuliang","family":"Yuan","sequence":"additional","affiliation":[{"name":"Institute of Physics National Laboratory for Condensed Matter Physics Chinese Academy of Sciences  Beijing 100190 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kewen","family":"Shi","sequence":"additional","affiliation":[{"name":"School of Integrated Circuit Science and Engineering Beihang University  Beijing 100191 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lunhua","family":"He","sequence":"additional","affiliation":[{"name":"Spallation Neutron Source Science Center  Dongguan 523803 China"},{"name":"Institute of Physics National Laboratory for Condensed Matter Physics Chinese Academy of Sciences  Beijing 100190 China"},{"name":"Songshan Lake Materials Laboratory  Dongguan 523808 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Bao","family":"Yuan","sequence":"additional","affiliation":[{"name":"Spallation Neutron Source Science Center  Dongguan 523803 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Liling","family":"Sun","sequence":"additional","affiliation":[{"name":"Institute of Physics National Laboratory for Condensed Matter Physics Chinese Academy of Sciences  Beijing 100190 China"},{"name":"Songshan Lake Materials Laboratory  Dongguan 523808 China"},{"name":"Department of Physics University of Chinese Academy of Sciences  Beijing 100190 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jing","family":"Guo","sequence":"additional","affiliation":[{"name":"Institute of Physics National Laboratory for Condensed Matter Physics Chinese Academy of Sciences  Beijing 100190 China"},{"name":"Songshan Lake Materials Laboratory  Dongguan 523808 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Pengyu","family":"Wang","sequence":"additional","affiliation":[{"name":"Institute of Physics National Laboratory for Condensed Matter Physics Chinese Academy of Sciences  Beijing 100190 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xianlei","family":"Sheng","sequence":"additional","affiliation":[{"name":"School of Physics Beihang University  Beijing 100191 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Weichang","family":"Hao","sequence":"additional","affiliation":[{"name":"School of Physics Beihang University  Beijing 100191 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yi","family":"Du","sequence":"additional","affiliation":[{"name":"School of Physics Beihang University  Beijing 100191 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qingzhen","family":"Huang","sequence":"additional","affiliation":[{"name":"Spallation Neutron Source Science Center  Dongguan 523803 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Cong","family":"Wang","sequence":"additional","affiliation":[{"name":"School of Integrated Circuit Science and Engineering Beihang University  Beijing 100191 China"},{"name":"National Key Lab of Spintronics Institute of International Innovation Beihang University  Yuhang Hangzhou 311115 China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2025,3,23]]},"reference":[{"key":"e_1_2_9_1_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41586-020-2197-9"},{"key":"e_1_2_9_2_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.1065389"},{"key":"e_1_2_9_3_1","doi-asserted-by":"publisher","DOI":"10.1038\/35081014"},{"key":"e_1_2_9_4_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41586-024-07125-5"},{"key":"e_1_2_9_5_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.1058371"},{"key":"e_1_2_9_6_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.mattod.2023.10.004"},{"key":"e_1_2_9_7_1","doi-asserted-by":"publisher","DOI":"10.1038\/nmat4566"},{"key":"e_1_2_9_8_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41928-020-0461-5"},{"key":"e_1_2_9_9_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41567-018-0051-x"},{"key":"e_1_2_9_10_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41563-023-01554-9"},{"key":"e_1_2_9_11_1","doi-asserted-by":"publisher","DOI":"10.1038\/nature02325"},{"key":"e_1_2_9_12_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41586-022-05461-y"},{"key":"e_1_2_9_13_1","doi-asserted-by":"publisher","DOI":"10.1126\/sciadv.adn0479"},{"key":"e_1_2_9_14_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41586-020-2211-2"},{"key":"e_1_2_9_15_1","doi-asserted-by":"publisher","DOI":"10.1038\/ncomms12519"},{"key":"e_1_2_9_16_1","doi-asserted-by":"publisher","DOI":"10.1038\/nmat4351"},{"key":"e_1_2_9_17_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41567-020-0927-4"},{"key":"e_1_2_9_18_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-018-05435-7"},{"key":"e_1_2_9_19_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-020-14325-w"},{"key":"e_1_2_9_20_1","doi-asserted-by":"publisher","DOI":"10.1126\/sciadv.aaw5639"},{"key":"e_1_2_9_21_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41563-021-01005-3"},{"key":"e_1_2_9_22_1","doi-asserted-by":"publisher","DOI":"10.1038\/nature15723"},{"key":"e_1_2_9_23_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41567-018-0064-5"},{"key":"e_1_2_9_24_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41586-022-04864-1"},{"key":"e_1_2_9_25_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41567-022-01645-5"},{"key":"e_1_2_9_26_1","doi-asserted-by":"publisher","DOI":"10.1038\/nphys4192"},{"key":"e_1_2_9_27_1","doi-asserted-by":"publisher","DOI":"10.1021\/ic300978x"},{"key":"e_1_2_9_28_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.201900947"},{"key":"e_1_2_9_29_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.201902502"},{"key":"e_1_2_9_30_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.95.184438"},{"key":"e_1_2_9_31_1","volume":"8","author":"Boldrin D.","year":"2018","journal-title":"Phys. Rev. X"},{"key":"e_1_2_9_32_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.96.024451"},{"key":"e_1_2_9_33_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.82.094417"},{"key":"e_1_2_9_34_1","doi-asserted-by":"publisher","DOI":"10.1016\/0038-1098(70)90579-X"},{"key":"e_1_2_9_35_1","doi-asserted-by":"publisher","DOI":"10.1016\/0021-9614(83)90031-9"},{"key":"e_1_2_9_36_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41567-019-0426-7"},{"key":"e_1_2_9_37_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41567-019-0451-6"},{"key":"e_1_2_9_38_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.67.060407"},{"key":"e_1_2_9_39_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.66.020406"},{"key":"e_1_2_9_40_1","doi-asserted-by":"publisher","DOI":"10.1143\/JPSJ.56.4047"},{"key":"e_1_2_9_41_1","doi-asserted-by":"publisher","DOI":"10.1143\/JPSJ.67.1748"},{"key":"e_1_2_9_42_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41586-022-05262-3"},{"key":"e_1_2_9_43_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41586-021-04028-7"},{"key":"e_1_2_9_44_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.84.3430"},{"key":"e_1_2_9_45_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.1064761"},{"key":"e_1_2_9_46_1","doi-asserted-by":"publisher","DOI":"10.1038\/nmat1357"},{"key":"e_1_2_9_47_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.106.195113"},{"key":"e_1_2_9_48_1","doi-asserted-by":"publisher","DOI":"10.1038\/nmat1353"},{"key":"e_1_2_9_49_1","doi-asserted-by":"publisher","DOI":"10.1038\/ncomms13842"},{"key":"e_1_2_9_50_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.61.2472"},{"key":"e_1_2_9_51_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.39.4828"},{"key":"e_1_2_9_52_1","doi-asserted-by":"publisher","DOI":"10.1002\/j.1538-7305.1967.tb01738.x"},{"key":"e_1_2_9_53_1","unstructured":"M.Holler S.Tam H.Castro R.Benson International 1989 Joint Conference on Neural Networks Washington DC USA June 1989."},{"key":"e_1_2_9_54_1","doi-asserted-by":"publisher","DOI":"10.1038\/nmat1860"},{"key":"e_1_2_9_55_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.90.014101"},{"key":"e_1_2_9_56_1","doi-asserted-by":"publisher","DOI":"10.1146\/annurev-matsci-070214-021008"},{"key":"e_1_2_9_57_1","doi-asserted-by":"publisher","DOI":"10.1038\/nmat4117"},{"key":"e_1_2_9_58_1","doi-asserted-by":"publisher","DOI":"10.1016\/0927-0256(96)00008-0"},{"key":"e_1_2_9_59_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.54.11169"},{"key":"e_1_2_9_60_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.47.558"},{"key":"e_1_2_9_61_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.77.3865"},{"key":"e_1_2_9_62_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.57.1505"}],"container-title":["Advanced Materials"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/advanced.onlinelibrary.wiley.com\/doi\/pdf\/10.1002\/adma.202420502","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2025,10,6]],"date-time":"2025-10-06T20:24:33Z","timestamp":1759782273000},"score":1,"resource":{"primary":{"URL":"https:\/\/advanced.onlinelibrary.wiley.com\/doi\/10.1002\/adma.202420502"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2025,3,23]]},"references-count":62,"journal-issue":{"issue":"18","published-print":{"date-parts":[[2025,5]]}},"alternative-id":["10.1002\/adma.202420502"],"URL":"https:\/\/doi.org\/10.1002\/adma.202420502","archive":["Portico"],"relation":{},"ISSN":["0935-9648","1521-4095"],"issn-type":[{"value":"0935-9648","type":"print"},{"value":"1521-4095","type":"electronic"}],"subject":[],"published":{"date-parts":[[2025,3,23]]},"assertion":[{"value":"2024-12-28","order":0,"name":"received","label":"Received","group":{"name":"publication_history","label":"Publication History"}},{"value":"2025-03-23","order":3,"name":"published","label":"Published","group":{"name":"publication_history","label":"Publication History"}}],"article-number":"2420502"}}