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Herein, a sacrificial template\u2010full solution method with both rough surface and high conductivity is described that can be applied to sandwich\u2010structured resistive pressure sensors. Transient absorption measurements demonstrate the significant increase of carrier lifetime (from 1.44 to 2.54\u00a0ns) induced by pressure, which directly evidenced the superior sensing mechanism of sidechain doped conjugated polymer. This sensor displayed low\u2010pressure detection limit of 0.7\u00a0Pa as well as a rapid response time of 18.8\u00a0ms, enabling multi\u2010mode motion analysis including wrist pulse, swallowing, finger bending, grabbing, and typing. Additionally, an intelligent vocal recognition system with convolutional neural networks is used which can achieve &gt;96% classification accuracy across diverse vocal profiles. This general approach is anticipated and enables a new direction for the development of pressure sensors.<\/jats:p>","DOI":"10.1002\/adma.202500077","type":"journal-article","created":{"date-parts":[[2025,4,9]],"date-time":"2025-04-09T02:09:11Z","timestamp":1744164551000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":10,"title":["Pressure Induced Molecular\u2010Arrangement and Charge\u2010Density Perturbance in Doped Polymer for Intelligent Motion and Vocal Recognitions"],"prefix":"10.1002","volume":"37","author":[{"given":"Huimin","family":"Lu","sequence":"first","affiliation":[{"name":"School of Microelectronics Shanghai University  Shanghai 201800 China"},{"name":"Sino\u2010Swiss Institute of Advanced Technology (SSIAT) Shanghai University  Shanghai 201899 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lei","family":"Zhang","sequence":"additional","affiliation":[{"name":"School of Microelectronics 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