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Concurrently, the harnessing of infrared (IR) light, which constitutes \u224850% of solar energy, has predominantly remained unexploited due to a pronounced contradiction between the utilization of IR light and CO<jats:sub>2<\/jats:sub> photoreduction. To break the above limitation, a dual\u2010plasmon resonance conductor with a metallic nature is designed, which realizes the synthesis of CO with 100% selectivity from infrared photothermal catalytic reduction of atmospheric carbon dioxide (CO<jats:sub>2<\/jats:sub>). Taking the Au particles loaded Cu<jats:sub>7<\/jats:sub>Te<jats:sub>4<\/jats:sub> nanowires as an example, the surface dual\u2010plasmon resonance coupling effect can optimize the three critical processes of CO<jats:sub>2<\/jats:sub> photoreduction, in which it is illustrated that the dual\u2010plasmon resonance effect lowers the thermodynamic reaction energy barrier, facilitating the selective generation of CO products. Consequently, the Au\u2010Cu<jats:sub>7<\/jats:sub>Te<jats:sub>4<\/jats:sub> nanowires manifest a CO evolution rate of \u22482.7\u00a0\u00b5mol g<jats:sup>\u22121<\/jats:sup> h<jats:sup>\u22121<\/jats:sup> with 100% selectivity for atmospheric CO<jats:sub>2<\/jats:sub> reduction driven by IR light, several times higher than that of the Cu<jats:sub>7<\/jats:sub>Te<jats:sub>4<\/jats:sub> nanowires.<\/jats:p>","DOI":"10.1002\/adma.202503021","type":"journal-article","created":{"date-parts":[[2025,6,1]],"date-time":"2025-06-01T22:31:51Z","timestamp":1748817111000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":33,"title":["Infrared Photothermal Catalytic Reduction of Atmospheric CO<sub>2<\/sub> Into CO with 100% Selectivity via Dual\u2010Plasmon Resonance Conductor"],"prefix":"10.1002","volume":"37","author":[{"given":"Mengqian","family":"Li","sequence":"first","affiliation":[{"name":"Key Laboratory of Synthetic and Biological Colloids Ministry of Education School of Chemical and Material Engineering Jiangnan University  Wuxi Jiangsu 214122 P. 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