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Advanced oxidation processes (AOPs) using solid oxidants offer a promising approach for decentralized freshwater production but are often limited by nonselective radical reactions that degrade both pollutants and background water constituents. Here, sonicated carbon nanotubes (CNTs) that efficiently activate peroxymonosulfate are demonstrated, enabling selective contaminant degradation via dual nonradical pathways\u2014singlet oxygen oxidation and direct electron transfer. Optimized sonication introduces catalytically active carbonyl (C\u2550O) groups on CNT surfaces while preserving their graphitic structure, ensuring rapid electron transfer. This approach achieves 2,4\u2010dichlorophenol removal, a common industrial and municipal pollutant, within 5\u00a0min at a record removal rate of 4.80\u00a0\u00b5mol\u00a0g<jats:sup>\u22121<\/jats:sup>\u00a0s<jats:sup>\u22121<\/jats:sup>. Furthermore, scalable CNT catalyst synthesis and integration into flat membrane and hollow fiber filtration devices, ensuring long\u2010term stability and efficient pollutant removal in natural river water, are demonstrated. By advancing selective CNT catalysts for AOPs, this work offers a scalable, sustainable solution for point\u2010of\u2010use freshwater production in real\u2010world applications.<\/jats:p>","DOI":"10.1002\/adma.202504618","type":"journal-article","created":{"date-parts":[[2025,5,21]],"date-time":"2025-05-21T03:51:11Z","timestamp":1747799471000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":15,"title":["Sonicated Carbon Nanotube Catalysts for Efficient Point\u2010of\u2010use Water Treatment"],"prefix":"10.1002","volume":"37","author":[{"given":"Xin","family":"Yang","sequence":"first","affiliation":[{"name":"School of Chemical and Biomolecular Engineering The University of Sydney  Darlington New South Wales 2006 Australia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Justin","family":"Prabowo","sequence":"additional","affiliation":[{"name":"School of Chemical and Biomolecular Engineering The University of Sydney  Darlington New South Wales 2006 Australia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jiaxiang","family":"Chen","sequence":"additional","affiliation":[{"name":"School of Chemical and Biomolecular Engineering The University of Sydney  Darlington New South Wales 2006 Australia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Fangxin","family":"She","sequence":"additional","affiliation":[{"name":"School of Chemical and Biomolecular Engineering The University of Sydney  Darlington New South Wales 2006 Australia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Leo","family":"Lai","sequence":"additional","affiliation":[{"name":"School of Chemical and Biomolecular Engineering The University of Sydney  Darlington New South Wales 2006 Australia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Fangzhou","family":"Liu","sequence":"additional","affiliation":[{"name":"School of Chemical and Biomolecular Engineering The University of Sydney  Darlington New South Wales 2006 Australia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhechao","family":"Hua","sequence":"additional","affiliation":[{"name":"Guangdong Provincial Key Laboratory of Environmental Pollution Control and Remediation Technology School of Environmental Science and Engineering Sun Yat\u2010Sen University  Guangzhou 510275 P. 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