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Herein, a novel CO\n                    <jats:sub>2<\/jats:sub>\n                    \u2010responsive smart wood scaffold that leverages non\u2010toxic CO\n                    <jats:sub>2<\/jats:sub>\n                    activation is developed to achieve highly efficient removal of carcinogenic natural organic matter (NOM) and broad\u2010spectrum microbial disinfection without requiring additional chemical agents. Unlike conventional water purification techniques that face a safety\u2010efficacy trade\u2010off, the multi\u2010stage CO\n                    <jats:sub>2<\/jats:sub>\n                    \u2010responsive wood scaffold offers exceptional tunability in NOM abatement across diverse environmental conditions, including variable water chemistry, NOM composition, high salinity, and real\u2010world water sources. The purified water meets stringent drinking water standards (e.g., UV\n                    <jats:sub>254<\/jats:sub>\n                    reduction, dissolved organic carbon removal, and bacterial elimination). It is found that the highly efficient NOM adsorption mainly originates from the strong and stable CO\n                    <jats:sub>2<\/jats:sub>\n                    \u2010triggered cation\u2212\u03c0 interaction between the scaffold surface and aromatic NOM groups, as revealed via high\u2010resolution mass spectrometry and direct intermolecular force measurements. This ecofriendly and contamination\u2010free CO\n                    <jats:sub>2<\/jats:sub>\n                    \u2010responsive strategy provides a transformative approach to overcoming secondary pollution challenges in water purification, offering a scalable and sustainable platform for environmental applications and beyond.\n                  <\/jats:p>","DOI":"10.1002\/adma.202505008","type":"journal-article","created":{"date-parts":[[2025,5,16]],"date-time":"2025-05-16T05:27:31Z","timestamp":1747373251000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":16,"title":["CO\n                    <sub>2<\/sub>\n                    \u2010Responsive Smart Wood Scaffold for Natural Organic Matter Removal without Secondary Pollution"],"prefix":"10.1002","volume":"37","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-8301-144X","authenticated-orcid":false,"given":"Lin","family":"Yang","sequence":"first","affiliation":[{"name":"Department of Chemical and Materials Engineering University of Alberta  Edmonton T6G 1H9 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yuanyuan","family":"Wang","sequence":"additional","affiliation":[{"name":"Department of Chemical and Materials Engineering University of Alberta  Edmonton T6G 1H9 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yongxiang","family":"Sun","sequence":"additional","affiliation":[{"name":"Department of Chemical and Materials Engineering University of Alberta  Edmonton T6G 1H9 Canada"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ruiquan","family":"Yu","sequence":"additional","affiliation":[{"name":"Institute of Environment and Ecology Tsinghua Shenzhen International Graduate School Tsinghua University  Shenzhen 518055 P. 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