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Membrane separation is a promising alternative, owing to its in simplicity, low energy consumption, and scalability. However, current membranes fail to achieve the selectivity and efficiency required for uranium capture. Herein, this study introduces a bioinspired graphene oxide\u2010red blood cells (GO\u2010RBC) membrane, that mimics vascular transport for ultra\u2010selective uranium extraction. In the innovative GO\u2010induced remodeling of red blood cell, hemoglobin (Hb) adsorbs onto the hydrophobic regions of GO and, phospholipids self\u2010assemble into concentric hydrophilic rings around Hb. This unique \u201cisland\u2010reef\u201d structure within the membrane channels forces ions to follow an S\u2010shaped path, thereby enhancing interactions with Hb. In addition, Hb catalytically reduces U(VI) to U(IV), enabling trapping of uranium while allowing competing ions to pass through. The membrane achieves an unprecedented U\/V selectivity (110.6), far outperforming current technologies. Moreover, the GO\u2010RBC membrane exhibited exceptional antifouling properties, mechanical robustness, and long\u2010term stability. This study provides a scalable, energy\u2010efficient solution for uranium extraction from seawater, further opening new pathways for the development of biomimetic membranes for application in resource recovery.<\/jats:p>","DOI":"10.1002\/adma.202509989","type":"journal-article","created":{"date-parts":[[2025,9,12]],"date-time":"2025-09-12T11:45:31Z","timestamp":1757677531000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":11,"title":["Vascular\u2010Mimetic 2D Membranes with Hemoglobin Catalysis for Efficient Uranium Extraction"],"prefix":"10.1002","volume":"38","author":[{"ORCID":"https:\/\/orcid.org\/0009-0000-8873-804X","authenticated-orcid":false,"given":"Siqi","family":"Han","sequence":"first","affiliation":[{"name":"MOE Frontiers Science Center for Rare Isotopes Lanzhou University  Lanzhou 730000 China"},{"name":"School of Nuclear Science and Technology Lanzhou University  Lanzhou 730000 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