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Typically, Zn plating proceeds via 2D growth along the six equivalent prismatic [ directions of the hexagonal close\u2010packed (HCP) Zn lattice, forming hexagonal platelets that promote dendrite formation. Here, an effective electrolyte engineering strategy is presented using rare\u2010earth ions to regulate Zn plating. Combined multiscale experimental analyses and computational modeling reveal that these ions preferentially adsorb onto the prismatic {} facets, suppressing lateral epitaxial growth of the basal (0002) planes. This redirects Zn plating toward an apparent screw dislocation\u2010driven growth along the [0001] axis. The resulting growth pathway, together with randomly oriented Zn nucleation, yields dense, uniform, and dendrite\u2010free Zn layers with markedly improved cycling stability and high depth\u2010of\u2010discharge operation, thereby challenging the prevailing assumption that dendrite suppression requires (0002)\u2010oriented growth parallel to the substrate. This work provides new mechanistic insights into Zn plating dynamics and establishes a scalable strategy for stable, dendrite\u2010free Zn anodes in next\u2010generation AZIBs.<\/jats:p>","DOI":"10.1002\/adma.202510906","type":"journal-article","created":{"date-parts":[[2025,9,30]],"date-time":"2025-09-30T13:03:40Z","timestamp":1759237420000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":17,"title":["Crystal Growth Engineering for Dendrite\u2010Free Zinc Metal Plating"],"prefix":"10.1002","volume":"38","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-5927-4730","authenticated-orcid":false,"given":"Guifang","family":"Zeng","sequence":"first","affiliation":[{"name":"Catalonia Institute for Energy Research (lREC) Sant Adri\u00e0 de Bes\u00f2s Barcelona 08930 Spain"},{"name":"Zhengzhou Research Institute Harbin Institute of Technology  Zhengzhou 450000 China"},{"name":"State Key Laboratory of Precision Welding &amp; Joining of Materials and Structures Harbin Institute of Technology Harbin 150001 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Sharona","family":"Horta","sequence":"additional","affiliation":[{"name":"Institute of Science and Technology Austria (ISTA)  Am Campus 1 Klosterneuburg 3400 Austria"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9145-7772","authenticated-orcid":false,"given":"Qing","family":"Sun","sequence":"additional","affiliation":[{"name":"Catalonia Institute for Energy Research (lREC) Sant Adri\u00e0 de Bes\u00f2s Barcelona 08930 Spain"},{"name":"Zhengzhou Research Institute Harbin Institute of Technology  Zhengzhou 450000 China"},{"name":"State Key Laboratory of Precision Welding &amp; Joining of Materials and Structures Harbin Institute of Technology Harbin 150001 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Malik Dilshad","family":"Khan","sequence":"additional","affiliation":[{"name":"Catalonia Institute for Energy Research (lREC) Sant Adri\u00e0 de Bes\u00f2s Barcelona 08930 Spain"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Maria","family":"Ib\u00e1\u00f1ez","sequence":"additional","affiliation":[{"name":"Institute of Science and Technology Austria (ISTA)  Am Campus 1 Klosterneuburg 3400 Austria"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yuhang","family":"Han","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Precision Welding &amp; Joining of Materials and Structures Harbin Institute of Technology Harbin 150001 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shang","family":"Wang","sequence":"additional","affiliation":[{"name":"Zhengzhou Research Institute Harbin Institute of Technology  Zhengzhou 450000 China"},{"name":"State Key Laboratory of Precision Welding &amp; Joining of Materials and Structures Harbin Institute of Technology Harbin 150001 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Longqiu","family":"Li","sequence":"additional","affiliation":[{"name":"Zhengzhou Research Institute Harbin Institute of Technology  Zhengzhou 450000 China"},{"name":"State Key Laboratory of Robotics and Systems Harbin Institute of Technology  Harbin 150001 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lijie","family":"Ci","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Precision Welding &amp; Joining of Materials and Structures Harbin Institute of Technology Harbin 150001 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yanhong","family":"Tian","sequence":"additional","affiliation":[{"name":"Zhengzhou Research Institute Harbin Institute of Technology  Zhengzhou 450000 China"},{"name":"State Key Laboratory of Precision Welding &amp; Joining of Materials and Structures Harbin Institute of Technology Harbin 150001 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-7533-3251","authenticated-orcid":false,"given":"Andreu","family":"Cabot","sequence":"additional","affiliation":[{"name":"Catalonia Institute for Energy Research (lREC) Sant Adri\u00e0 de Bes\u00f2s Barcelona 08930 Spain"},{"name":"ICREA Pg. 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